A single optically detectable tumbling spin in silicon

Fuente: arXiv
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Autores principales: Cache, Félix, Baron, Yoann, Lefaucher, Baptiste, Jager, Jean-Baptiste, Mazen, Frédéric, Milési, Frédéric, Kerdilès, Sébastien, Robert-Philip, Isabelle, Gérard, Jean-Michel, Cassabois, Guillaume, Jacques, Vincent, Dréau, Anaïs
Formato: Preprint
Publicado: 2025
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author Cache, Félix
Baron, Yoann
Lefaucher, Baptiste
Jager, Jean-Baptiste
Mazen, Frédéric
Milési, Frédéric
Kerdilès, Sébastien
Robert-Philip, Isabelle
Gérard, Jean-Michel
Cassabois, Guillaume
Jacques, Vincent
Dréau, Anaïs
author_facet Cache, Félix
Baron, Yoann
Lefaucher, Baptiste
Jager, Jean-Baptiste
Mazen, Frédéric
Milési, Frédéric
Kerdilès, Sébastien
Robert-Philip, Isabelle
Gérard, Jean-Michel
Cassabois, Guillaume
Jacques, Vincent
Dréau, Anaïs
contents We demonstrate single spin spectroscopy of a fluorescent tumbling defect in silicon called the G center, behaving as a pseudo-molecule randomly reorienting itself in the crystalline matrix. Using high-resolution spin spectroscopy, we reveal a fine magnetic structure resulting from the spin principal axes jumping between discrete orientations in the crystal. Modeling the atomic reorientation of the defect shows that spin tumbling induces variations in the coupling to the microwave magnetic field, enabling position-dependent Rabi frequencies to be detected in coherent spin control experiments. By virtue of its pseudo-molecule configuration, the G center in silicon is a unique quantum system to investigate the mutual interaction between optical, spin and rotation properties in a highly versatile material.
format Preprint
id arxiv_https___arxiv_org_abs_2510_15590
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle A single optically detectable tumbling spin in silicon
Cache, Félix
Baron, Yoann
Lefaucher, Baptiste
Jager, Jean-Baptiste
Mazen, Frédéric
Milési, Frédéric
Kerdilès, Sébastien
Robert-Philip, Isabelle
Gérard, Jean-Michel
Cassabois, Guillaume
Jacques, Vincent
Dréau, Anaïs
Quantum Physics
We demonstrate single spin spectroscopy of a fluorescent tumbling defect in silicon called the G center, behaving as a pseudo-molecule randomly reorienting itself in the crystalline matrix. Using high-resolution spin spectroscopy, we reveal a fine magnetic structure resulting from the spin principal axes jumping between discrete orientations in the crystal. Modeling the atomic reorientation of the defect shows that spin tumbling induces variations in the coupling to the microwave magnetic field, enabling position-dependent Rabi frequencies to be detected in coherent spin control experiments. By virtue of its pseudo-molecule configuration, the G center in silicon is a unique quantum system to investigate the mutual interaction between optical, spin and rotation properties in a highly versatile material.
title A single optically detectable tumbling spin in silicon
topic Quantum Physics
url https://arxiv.org/abs/2510.15590