Chiral light from an emitter coupled to an achiral particle via the Purcell effect

Fuente: arXiv
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Auteurs principaux: Xuan, Yining, Miyazaki, Daito, Ishikawa, Yuki, Sadgrove, Mark
Format: Preprint
Publié: 2025
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author Xuan, Yining
Miyazaki, Daito
Ishikawa, Yuki
Sadgrove, Mark
author_facet Xuan, Yining
Miyazaki, Daito
Ishikawa, Yuki
Sadgrove, Mark
contents We demonstrate that non-chiral nanoparticles can produce chiral light when point emitters are coupled to their surface plasmon modes (SPMs) under certain conditions. Chiral emission arises from asymmetrical plasmon mode propagation from the source combined with the spin-momentum locked nature of the SPMs. The Purcell regime of cavity quantum electrodynamics (QED) ensures that radiation from the coupled mode dominates over that from the emitter itself, giving rise to photons with a circularly polarized component -- i.e. chiral light. We experimentally demonstrate this effect using electron beam-induced cathode luminescence from a gold nanorod, coupling it evanescently to a nanofiber probe which also supports spin-momentum locked light. This converts the net spin of the emission into a net directionality of propagation in the fiber modes.
format Preprint
id arxiv_https___arxiv_org_abs_2510_18166
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Chiral light from an emitter coupled to an achiral particle via the Purcell effect
Xuan, Yining
Miyazaki, Daito
Ishikawa, Yuki
Sadgrove, Mark
Quantum Physics
We demonstrate that non-chiral nanoparticles can produce chiral light when point emitters are coupled to their surface plasmon modes (SPMs) under certain conditions. Chiral emission arises from asymmetrical plasmon mode propagation from the source combined with the spin-momentum locked nature of the SPMs. The Purcell regime of cavity quantum electrodynamics (QED) ensures that radiation from the coupled mode dominates over that from the emitter itself, giving rise to photons with a circularly polarized component -- i.e. chiral light. We experimentally demonstrate this effect using electron beam-induced cathode luminescence from a gold nanorod, coupling it evanescently to a nanofiber probe which also supports spin-momentum locked light. This converts the net spin of the emission into a net directionality of propagation in the fiber modes.
title Chiral light from an emitter coupled to an achiral particle via the Purcell effect
topic Quantum Physics
url https://arxiv.org/abs/2510.18166