Soft Phonon Charge-Density Wave Formation in the Kagome Metal KV$_3$Sb$_5$

Fuente: arXiv
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Autori principali: Wang, Yifan, Xu, Chenchao, Wu, Zhimian, Rao, Huachen, Shan, Zhaoyang, Liu, Yi, Cao, Guanghan, Smidman, Michael, Shi, Ming, Yuan, Huiqiu, Wu, Tao, Chen, Xianhui, Cao, Chao, Song, Yu
Natura: Preprint
Pubblicazione: 2025
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author Wang, Yifan
Xu, Chenchao
Wu, Zhimian
Rao, Huachen
Shan, Zhaoyang
Liu, Yi
Cao, Guanghan
Smidman, Michael
Shi, Ming
Yuan, Huiqiu
Wu, Tao
Chen, Xianhui
Cao, Chao
Song, Yu
author_facet Wang, Yifan
Xu, Chenchao
Wu, Zhimian
Rao, Huachen
Shan, Zhaoyang
Liu, Yi
Cao, Guanghan
Smidman, Michael
Shi, Ming
Yuan, Huiqiu
Wu, Tao
Chen, Xianhui
Cao, Chao
Song, Yu
contents A range of of unusual emergent behaviors have been reported in the charge-density wave (CDW) state of the $A$V$_3$Sb$_5$ ($A=~$K, Rb, Cs) kagome metals, including a CDW formation process without soft phonons, which points to an unconventional CDW mechanism. Here, we use inelastic x-ray scattering to show that the CDW in KV$_3$Sb$_5$ forms via phonons that soften to zero energy at the CDW ordering vector ($L$-point) around $T_{\rm CDW}=78$~K. The intensity of soft phonons exhibit a remarkable in-plane anisotropy, extending over a much larger momentum range along $L$-$A$ relative to $L$-$H$, which leads to diffuse scattering common among $A$V$_3$Sb$_5$. Using first-principles calculations, we find that the momentum-dependent electron-phonon coupling (EPC) is peaked at $L$ and exhibits the same in-plane anisotropy as the phonon softening. Conversely, the electronic susceptibility is not peaked at $L$ and shows the opposite in-plane anisotropy. Our findings favor momentum-dependent EPC as the driving mechanism of the CDW in KV$_3$Sb$_5$, with a CDW formation process similar to that of transition metal dichalcogenides.
format Preprint
id arxiv_https___arxiv_org_abs_2510_20230
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Soft Phonon Charge-Density Wave Formation in the Kagome Metal KV$_3$Sb$_5$
Wang, Yifan
Xu, Chenchao
Wu, Zhimian
Rao, Huachen
Shan, Zhaoyang
Liu, Yi
Cao, Guanghan
Smidman, Michael
Shi, Ming
Yuan, Huiqiu
Wu, Tao
Chen, Xianhui
Cao, Chao
Song, Yu
Superconductivity
Strongly Correlated Electrons
A range of of unusual emergent behaviors have been reported in the charge-density wave (CDW) state of the $A$V$_3$Sb$_5$ ($A=~$K, Rb, Cs) kagome metals, including a CDW formation process without soft phonons, which points to an unconventional CDW mechanism. Here, we use inelastic x-ray scattering to show that the CDW in KV$_3$Sb$_5$ forms via phonons that soften to zero energy at the CDW ordering vector ($L$-point) around $T_{\rm CDW}=78$~K. The intensity of soft phonons exhibit a remarkable in-plane anisotropy, extending over a much larger momentum range along $L$-$A$ relative to $L$-$H$, which leads to diffuse scattering common among $A$V$_3$Sb$_5$. Using first-principles calculations, we find that the momentum-dependent electron-phonon coupling (EPC) is peaked at $L$ and exhibits the same in-plane anisotropy as the phonon softening. Conversely, the electronic susceptibility is not peaked at $L$ and shows the opposite in-plane anisotropy. Our findings favor momentum-dependent EPC as the driving mechanism of the CDW in KV$_3$Sb$_5$, with a CDW formation process similar to that of transition metal dichalcogenides.
title Soft Phonon Charge-Density Wave Formation in the Kagome Metal KV$_3$Sb$_5$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2510.20230