Polymorphic self-poisoning in poly(lactic acid): a new phenomenon in polymer crystallization

Fuente: arXiv
Saved in:
Bibliographic Details
Main Authors: Yang, Shu-Gui, Zeng, Xiang-bing, Liu, Feng, Ungar, Goran
Format: Preprint
Published: 2025
Subjects:
Online Access:
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866908607031803904
author Yang, Shu-Gui
Zeng, Xiang-bing
Liu, Feng
Ungar, Goran
author_facet Yang, Shu-Gui
Zeng, Xiang-bing
Liu, Feng
Ungar, Goran
contents Self-poisoning (SP) is ubiquitous in polymer crystallization, but has so far manifested itself visibly only as minima in growth rate vs. temperature in either monodisperse systems where e.g. unstable folded chains obstruct crystallization of stable extended chains, or in periodically segmented chains where unstable stems with n-1 segments disturb deposition of stable stems with n segments. Here we report a new type of self-poisoning found in poly(lactic acid) (PLA), where a less stable crystal form (alpha') disturbs growth of the stable form (alpha). While alpha requires strict up-down order of the polar chains, alpha' does not, hence is kinetically favoured. Unexpectedly, below the temperature of the growth rate minimum the lamellar thickness increases rather than drops, as in all other reported cases of polymer crystallization with decreasing temperature. A growth rate equation model is developed, giving good match with experiments, but revealing an unexpectedly low fold surface free energy of alpha' form. Due to SP of alpha, most practical fast-cooling processing gives the low-modulus alpha'-form grown close to Tg, explaining generally poor mechanical properties of the bio-friendly PLA.
format Preprint
id arxiv_https___arxiv_org_abs_2510_20370
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Polymorphic self-poisoning in poly(lactic acid): a new phenomenon in polymer crystallization
Yang, Shu-Gui
Zeng, Xiang-bing
Liu, Feng
Ungar, Goran
Soft Condensed Matter
Self-poisoning (SP) is ubiquitous in polymer crystallization, but has so far manifested itself visibly only as minima in growth rate vs. temperature in either monodisperse systems where e.g. unstable folded chains obstruct crystallization of stable extended chains, or in periodically segmented chains where unstable stems with n-1 segments disturb deposition of stable stems with n segments. Here we report a new type of self-poisoning found in poly(lactic acid) (PLA), where a less stable crystal form (alpha') disturbs growth of the stable form (alpha). While alpha requires strict up-down order of the polar chains, alpha' does not, hence is kinetically favoured. Unexpectedly, below the temperature of the growth rate minimum the lamellar thickness increases rather than drops, as in all other reported cases of polymer crystallization with decreasing temperature. A growth rate equation model is developed, giving good match with experiments, but revealing an unexpectedly low fold surface free energy of alpha' form. Due to SP of alpha, most practical fast-cooling processing gives the low-modulus alpha'-form grown close to Tg, explaining generally poor mechanical properties of the bio-friendly PLA.
title Polymorphic self-poisoning in poly(lactic acid): a new phenomenon in polymer crystallization
topic Soft Condensed Matter
url https://arxiv.org/abs/2510.20370