Development of a 10.8-eV Tabletop Femtosecond Laser with Tunable Polarization for High-Resolution Angle-Resolved Photoemission Spectroscopy

Fuente: arXiv
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Autori principali: Gao, Jisong, Zhao, Qiaoxiao, Liu, Wenbo, Li, Dong, Gao, Zhicheng, Zhou, Yudian, Hu, Xuegao, Cai, Zhihao, Li, Zhilin, Shi, Youguo, Cheng, Peng, Liu, Zhaojun, Chen, Lan, Wu, Kehui, Zhao, Zhigang, Feng, Baojie
Natura: Preprint
Pubblicazione: 2025
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author Gao, Jisong
Zhao, Qiaoxiao
Liu, Wenbo
Li, Dong
Gao, Zhicheng
Zhou, Yudian
Hu, Xuegao
Cai, Zhihao
Li, Zhilin
Shi, Youguo
Cheng, Peng
Liu, Zhaojun
Chen, Lan
Wu, Kehui
Zhao, Zhigang
Feng, Baojie
author_facet Gao, Jisong
Zhao, Qiaoxiao
Liu, Wenbo
Li, Dong
Gao, Zhicheng
Zhou, Yudian
Hu, Xuegao
Cai, Zhihao
Li, Zhilin
Shi, Youguo
Cheng, Peng
Liu, Zhaojun
Chen, Lan
Wu, Kehui
Zhao, Zhigang
Feng, Baojie
contents The development of extreme ultraviolet sources is critical for advancing angleresolved photoemission spectroscopy (ARPES), a powerful technique for probing the electronic structure of materials. Here, we report the construction of a tabletop 10.8-eV femtosecond laser through cascaded third-harmonic generation, which operates at a repetition rate of 1 MHz and delivers a photon flux of approximately 1012 photons/s. The system achieves a high energy resolution of approximately 11.8 meV and tunable polarization. This flexibility enables detailed studies of orbitaland (pseudo)spin characteristics in quantum materials. We demonstrate the capabilities of this laser-ARPES system by investigating several prototypical materials, showcasing its potential for elucidating complex phenomena in quantum materials.
format Preprint
id arxiv_https___arxiv_org_abs_2510_24158
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Development of a 10.8-eV Tabletop Femtosecond Laser with Tunable Polarization for High-Resolution Angle-Resolved Photoemission Spectroscopy
Gao, Jisong
Zhao, Qiaoxiao
Liu, Wenbo
Li, Dong
Gao, Zhicheng
Zhou, Yudian
Hu, Xuegao
Cai, Zhihao
Li, Zhilin
Shi, Youguo
Cheng, Peng
Liu, Zhaojun
Chen, Lan
Wu, Kehui
Zhao, Zhigang
Feng, Baojie
Materials Science
Optics
The development of extreme ultraviolet sources is critical for advancing angleresolved photoemission spectroscopy (ARPES), a powerful technique for probing the electronic structure of materials. Here, we report the construction of a tabletop 10.8-eV femtosecond laser through cascaded third-harmonic generation, which operates at a repetition rate of 1 MHz and delivers a photon flux of approximately 1012 photons/s. The system achieves a high energy resolution of approximately 11.8 meV and tunable polarization. This flexibility enables detailed studies of orbitaland (pseudo)spin characteristics in quantum materials. We demonstrate the capabilities of this laser-ARPES system by investigating several prototypical materials, showcasing its potential for elucidating complex phenomena in quantum materials.
title Development of a 10.8-eV Tabletop Femtosecond Laser with Tunable Polarization for High-Resolution Angle-Resolved Photoemission Spectroscopy
topic Materials Science
Optics
url https://arxiv.org/abs/2510.24158