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Detalles Bibliográficos
Autores principales: Das, Arpita, Tao, Albert Li, Fernley, Luke M., von Gierke, Fritz, Gregory, Philip D., Cornish, Simon L., Hutson, Jeremy M., Vexiau, Romain, Dulieu, Olivier
Formato: Preprint
Publicado: 2025
Materias:
Acceso en línea:https://arxiv.org/abs/2510.24660
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  • Using an ultracold gas of $^{87}$Rb$^{133}$Cs molecules, we perform hyperfine-resolved spectroscopy of transitions from the vibronic ground state to the lowest rovibrational states of the electronic state $\mathrm{b}\,^3Π_0$, as a function of magnetic field. These transitions are spin forbidden, resulting in narrow linewidths, and feature near-diagonal Franck-Condon factors. We develop a model of the hyperfine and Zeeman structure that includes coupling between the $0^+$ and $0^-$ components of $\mathrm{b}\,^3Π_0$. We fit the spectra to obtain rotational and hyperfine coupling constants. We measure transition dipole moments associated with specific transitions by directly observing Rabi oscillations as a function of a resonant laser pulse duration. Using resonant $π$ pulses, we prepare molecules in the electronically excited state and directly measure the spontaneous emission rate.