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Main Authors: Saykin, David R., Jiang, Qianni, Liu, Zhaoyu, Shekhar, Chandra, Felser, Claudia, Chu, Jiun-Haw, Kapitulnik, Aharon
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2510.26010
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author Saykin, David R.
Jiang, Qianni
Liu, Zhaoyu
Shekhar, Chandra
Felser, Claudia
Chu, Jiun-Haw
Kapitulnik, Aharon
author_facet Saykin, David R.
Jiang, Qianni
Liu, Zhaoyu
Shekhar, Chandra
Felser, Claudia
Chu, Jiun-Haw
Kapitulnik, Aharon
contents We report high resolution polar Kerr effect measurements on CsV3Sb5 and ScV6Sn6 single crystals in search for signatures of spontaneous polar Kerr effect (PKE) below the charge order transitions of these materials. Utilizing two separate zero-area loop Sagnac interferometers operating at 1550 nm and 830 nm wavelengths, we studied the temperature dependence of possible PKE after training with magnetic field. While a finite field Kerr measurement yielded optical rotation expected from the Pauli susceptibility of the itinerant carriers, no signal was detected at zero-field to within the noise floor limit of the apparatus of below $\sim$100 nanoradians. Simultaneous coherent reflection measurements confirm the sharpness of the charge order transition in the same optical volume as the Kerr measurements. Application of strain to reveal a hidden flux-ordered magnetic state did not result in a finite Kerr effect.
format Preprint
id arxiv_https___arxiv_org_abs_2510_26010
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle High Resolution Polar Kerr Effect Studies of Cs3Sb5 and ScV6Sn6 Below the Charge Order Transition
Saykin, David R.
Jiang, Qianni
Liu, Zhaoyu
Shekhar, Chandra
Felser, Claudia
Chu, Jiun-Haw
Kapitulnik, Aharon
Strongly Correlated Electrons
We report high resolution polar Kerr effect measurements on CsV3Sb5 and ScV6Sn6 single crystals in search for signatures of spontaneous polar Kerr effect (PKE) below the charge order transitions of these materials. Utilizing two separate zero-area loop Sagnac interferometers operating at 1550 nm and 830 nm wavelengths, we studied the temperature dependence of possible PKE after training with magnetic field. While a finite field Kerr measurement yielded optical rotation expected from the Pauli susceptibility of the itinerant carriers, no signal was detected at zero-field to within the noise floor limit of the apparatus of below $\sim$100 nanoradians. Simultaneous coherent reflection measurements confirm the sharpness of the charge order transition in the same optical volume as the Kerr measurements. Application of strain to reveal a hidden flux-ordered magnetic state did not result in a finite Kerr effect.
title High Resolution Polar Kerr Effect Studies of Cs3Sb5 and ScV6Sn6 Below the Charge Order Transition
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2510.26010