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Main Authors: Chai, Hua, Cheng, Zhenyu, Hu, Qinxin, Huang, Zhongbing, Hu, Xiang, Tian, Xuedong, Du, Liang
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2510.26288
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author Chai, Hua
Cheng, Zhenyu
Hu, Qinxin
Huang, Zhongbing
Hu, Xiang
Tian, Xuedong
Du, Liang
author_facet Chai, Hua
Cheng, Zhenyu
Hu, Qinxin
Huang, Zhongbing
Hu, Xiang
Tian, Xuedong
Du, Liang
contents We investigate the nonequilibrium dynamics of charge density waves in a pumped one-dimensional Hubbard superlattice with staggered onsite Coulomb interactions at half-filling, using time-dependent exact diagonalization. In equilibrium, the system exhibits commensurate charge correlations consistent with the superlattice periodicity. Under laser excitation, the charge correlation function exhibits distinct behaviors across four representative frequencies, spanning both linear and nonlinear optical regimes. Notably, we observe a laser-induced commensurate-to-incommensurate transition in the charge order, manifested by a shift in the peak wavevector of the charge structure factor. This transition is driven by sublattice-selective doublon-holon dynamics, where the laser frequency and intensity determine whether excitations predominantly destabilize the charge order on the weakly or strongly interacting sublattice. Our analysis of the excitation spectrum and site-resolved correlation dynamics reveals the underlying mechanisms of this transition. These results suggest a promising optical strategy for controlling charge order in superlattice-based quantum materials.
format Preprint
id arxiv_https___arxiv_org_abs_2510_26288
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Laser-Induced Commensurate-Incommensurate Transition of Charge Order in a Hubbard Superlattice
Chai, Hua
Cheng, Zhenyu
Hu, Qinxin
Huang, Zhongbing
Hu, Xiang
Tian, Xuedong
Du, Liang
Strongly Correlated Electrons
We investigate the nonequilibrium dynamics of charge density waves in a pumped one-dimensional Hubbard superlattice with staggered onsite Coulomb interactions at half-filling, using time-dependent exact diagonalization. In equilibrium, the system exhibits commensurate charge correlations consistent with the superlattice periodicity. Under laser excitation, the charge correlation function exhibits distinct behaviors across four representative frequencies, spanning both linear and nonlinear optical regimes. Notably, we observe a laser-induced commensurate-to-incommensurate transition in the charge order, manifested by a shift in the peak wavevector of the charge structure factor. This transition is driven by sublattice-selective doublon-holon dynamics, where the laser frequency and intensity determine whether excitations predominantly destabilize the charge order on the weakly or strongly interacting sublattice. Our analysis of the excitation spectrum and site-resolved correlation dynamics reveals the underlying mechanisms of this transition. These results suggest a promising optical strategy for controlling charge order in superlattice-based quantum materials.
title Laser-Induced Commensurate-Incommensurate Transition of Charge Order in a Hubbard Superlattice
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2510.26288