Towards intense single-digit attosecond pulses with a 100-mJ-class mid-infrared sub-cycle laser

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Hauptverfasser: Nishimiya, Kaito, Rajpoot, Rambabu, Takahashi, Eiji J
Format: Preprint
Veröffentlicht: 2025
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author Nishimiya, Kaito
Rajpoot, Rambabu
Takahashi, Eiji J
author_facet Nishimiya, Kaito
Rajpoot, Rambabu
Takahashi, Eiji J
contents The duration of isolated attosecond pulses created via high-order harmonic generation is determined by the number of optical cycles in the driving laser. Achieving shorter attosecond soft X-ray pulses requires minimizing the number of cycles while maintaining a high pulse energy. Here, we demonstrate a carrier-envelope-phase-stable, 100-mJ-class sub-cycle mid-infrared laser that produces a supercontinuum coherent soft X-ray with unprecedented bandwidth. The system delivers 50-mJ, 6.7-fs (0.88-cycle) pulses at a center wavelength of 2.26 $μ$m - over two orders of magnitude more energetic than any previous sub-cycle laser. We applied the system to high-order harmonic generation and compared the results to simulations based on the three-dimensional time-dependent Schrödinger equation to identify unique features of sub-cycle lasers. This work represents a decisive step toward high-energy half-cycle lasers and high-energy single-digit attosecond soft X-ray pulses that can be used to probe matter and light-matter interactions at previously inaccessible temporal resolutions.
format Preprint
id arxiv_https___arxiv_org_abs_2510_27096
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Towards intense single-digit attosecond pulses with a 100-mJ-class mid-infrared sub-cycle laser
Nishimiya, Kaito
Rajpoot, Rambabu
Takahashi, Eiji J
Optics
Applied Physics
Atomic and Molecular Clusters
The duration of isolated attosecond pulses created via high-order harmonic generation is determined by the number of optical cycles in the driving laser. Achieving shorter attosecond soft X-ray pulses requires minimizing the number of cycles while maintaining a high pulse energy. Here, we demonstrate a carrier-envelope-phase-stable, 100-mJ-class sub-cycle mid-infrared laser that produces a supercontinuum coherent soft X-ray with unprecedented bandwidth. The system delivers 50-mJ, 6.7-fs (0.88-cycle) pulses at a center wavelength of 2.26 $μ$m - over two orders of magnitude more energetic than any previous sub-cycle laser. We applied the system to high-order harmonic generation and compared the results to simulations based on the three-dimensional time-dependent Schrödinger equation to identify unique features of sub-cycle lasers. This work represents a decisive step toward high-energy half-cycle lasers and high-energy single-digit attosecond soft X-ray pulses that can be used to probe matter and light-matter interactions at previously inaccessible temporal resolutions.
title Towards intense single-digit attosecond pulses with a 100-mJ-class mid-infrared sub-cycle laser
topic Optics
Applied Physics
Atomic and Molecular Clusters
url https://arxiv.org/abs/2510.27096