Deterministic generation of single B centers in hBN by one-to-one conversion from UV centers

Fuente: arXiv
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Autori principali: Marcos, Andrés Núñez, Arnold, Christophe, Barjon, Julien, Buil, Stéphanie, Hermier, Jean-Pierre, Delteil, Aymeric
Natura: Preprint
Pubblicazione: 2025
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author Marcos, Andrés Núñez
Arnold, Christophe
Barjon, Julien
Buil, Stéphanie
Hermier, Jean-Pierre
Delteil, Aymeric
author_facet Marcos, Andrés Núñez
Arnold, Christophe
Barjon, Julien
Buil, Stéphanie
Hermier, Jean-Pierre
Delteil, Aymeric
contents Among the variety of quantum emitters in hexagonal boron nitride (hBN), blue-emitting color centers, or B centers, have gathered a particular interest owing to their excellent quantum optical properties. Moreover, the fact that they can be locally activated by an electron beam makes them suitable for top-down integration in photonic devices. However, in the absence of a real-time monitoring technique sensitive to individual emitters, the activation process is stochastic in the number of emitters, and its mechanism is under debate. Here, we implement an in-situ cathodoluminescence monitoring setup capable of detecting individual quantum emitters in the blue and ultraviolet (UV) range. We demonstrate that the activation of individual B centers is spatially and temporally correlated with the deactivation of individual UV centers emitting at 4.1 eV, which are ubiquitous in hBN. We then make use of the ability to detect individual B center activation events to demonstrate the controlled creation of an array with only one emitter per irradiation site. Additionally, we demonstrate a symmetric technique for heralded selective deactivation of individual emitters. Our results provide insights into the microscopic structure and activation mechanism of B centers, as well as versatile techniques for their deterministic integration.
format Preprint
id arxiv_https___arxiv_org_abs_2511_02465
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Deterministic generation of single B centers in hBN by one-to-one conversion from UV centers
Marcos, Andrés Núñez
Arnold, Christophe
Barjon, Julien
Buil, Stéphanie
Hermier, Jean-Pierre
Delteil, Aymeric
Other Condensed Matter
Optics
Quantum Physics
Among the variety of quantum emitters in hexagonal boron nitride (hBN), blue-emitting color centers, or B centers, have gathered a particular interest owing to their excellent quantum optical properties. Moreover, the fact that they can be locally activated by an electron beam makes them suitable for top-down integration in photonic devices. However, in the absence of a real-time monitoring technique sensitive to individual emitters, the activation process is stochastic in the number of emitters, and its mechanism is under debate. Here, we implement an in-situ cathodoluminescence monitoring setup capable of detecting individual quantum emitters in the blue and ultraviolet (UV) range. We demonstrate that the activation of individual B centers is spatially and temporally correlated with the deactivation of individual UV centers emitting at 4.1 eV, which are ubiquitous in hBN. We then make use of the ability to detect individual B center activation events to demonstrate the controlled creation of an array with only one emitter per irradiation site. Additionally, we demonstrate a symmetric technique for heralded selective deactivation of individual emitters. Our results provide insights into the microscopic structure and activation mechanism of B centers, as well as versatile techniques for their deterministic integration.
title Deterministic generation of single B centers in hBN by one-to-one conversion from UV centers
topic Other Condensed Matter
Optics
Quantum Physics
url https://arxiv.org/abs/2511.02465