Nonadiabatic corrections to electric quadrupole transition rates in H$_2$

Fuente: arXiv
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Autori principali: Pachucki, Krzysztof, Siłkowski, Michał
Natura: Preprint
Pubblicazione: 2025
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author Pachucki, Krzysztof
Siłkowski, Michał
author_facet Pachucki, Krzysztof
Siłkowski, Michał
contents We derive formulas and perform calculations of nonadiabatic corrections to rates of electric quadrupole transitions in the hydrogen molecule. These corrections can be represented in terms of the quadrupole moment curve $D^{(1)}(R)$, similarly to the Born-Oppenheimer one, $D^{(0)}(R)$, derived originally by Wolniewicz. Numerical results change E2 transition rates for the fundamental band by as much as 0.4 - 12\% depending on rotational quantum numbers.
format Preprint
id arxiv_https___arxiv_org_abs_2511_02716
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Nonadiabatic corrections to electric quadrupole transition rates in H$_2$
Pachucki, Krzysztof
Siłkowski, Michał
Atomic Physics
Chemical Physics
We derive formulas and perform calculations of nonadiabatic corrections to rates of electric quadrupole transitions in the hydrogen molecule. These corrections can be represented in terms of the quadrupole moment curve $D^{(1)}(R)$, similarly to the Born-Oppenheimer one, $D^{(0)}(R)$, derived originally by Wolniewicz. Numerical results change E2 transition rates for the fundamental band by as much as 0.4 - 12\% depending on rotational quantum numbers.
title Nonadiabatic corrections to electric quadrupole transition rates in H$_2$
topic Atomic Physics
Chemical Physics
url https://arxiv.org/abs/2511.02716