Niobium's intrinsic coherence length and penetration depth revisited using low-energy muon spin spectroscopy and secondary-ion mass spectrometry

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Auteurs principaux: McFadden, Ryan M. L., Angle, Jonathan W., Lechner, Eric M., Kelley, Michael J., Reece, Charles E., Coble, Matthew A., Prokscha, Thomas, Salman, Zaher, Suter, Andreas, Junginger, Tobias
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Publié: 2025
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author McFadden, Ryan M. L.
Angle, Jonathan W.
Lechner, Eric M.
Kelley, Michael J.
Reece, Charles E.
Coble, Matthew A.
Prokscha, Thomas
Salman, Zaher
Suter, Andreas
Junginger, Tobias
author_facet McFadden, Ryan M. L.
Angle, Jonathan W.
Lechner, Eric M.
Kelley, Michael J.
Reece, Charles E.
Coble, Matthew A.
Prokscha, Thomas
Salman, Zaher
Suter, Andreas
Junginger, Tobias
contents We report direct, simultaneous measurements of the London penetration depth ($λ_L$) and Bardeen-Cooper-Schrieffer (BCS) coherence length ($ξ_0$) in oxygen-doped niobium, with impurity concentrations spanning the "clean" to "dirty" limits. Two depth-resolved techniques - low-energy muon spin spectroscopy (LE-$μ$SR) and secondary-ion mass spectrometry (SIMS) - were used to quantify the element's Meissner screening profiles, analyzed within a framework that accounts for nonlocal electrodynamics. The analysis indicates intrinsic length scales of $λ_L = 29.1(10)$ nm and $ξ_0 = 39.9(25)$ nm, corresponding to a Ginzburg-Landau (GL) parameter of $κ= 0.70(5)$. The obtained $λ_L$ and $κ$ values, accurately quantified at the nanoscale, are smaller than values commonly used in applications and modeling, and indicate that clean niobium lies at the boundary between type-I and type-II superconductivity, supporting the contemporary view that its intrinsic state may be type-I.
format Preprint
id arxiv_https___arxiv_org_abs_2511_02913
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Niobium's intrinsic coherence length and penetration depth revisited using low-energy muon spin spectroscopy and secondary-ion mass spectrometry
McFadden, Ryan M. L.
Angle, Jonathan W.
Lechner, Eric M.
Kelley, Michael J.
Reece, Charles E.
Coble, Matthew A.
Prokscha, Thomas
Salman, Zaher
Suter, Andreas
Junginger, Tobias
Superconductivity
Mesoscale and Nanoscale Physics
Materials Science
We report direct, simultaneous measurements of the London penetration depth ($λ_L$) and Bardeen-Cooper-Schrieffer (BCS) coherence length ($ξ_0$) in oxygen-doped niobium, with impurity concentrations spanning the "clean" to "dirty" limits. Two depth-resolved techniques - low-energy muon spin spectroscopy (LE-$μ$SR) and secondary-ion mass spectrometry (SIMS) - were used to quantify the element's Meissner screening profiles, analyzed within a framework that accounts for nonlocal electrodynamics. The analysis indicates intrinsic length scales of $λ_L = 29.1(10)$ nm and $ξ_0 = 39.9(25)$ nm, corresponding to a Ginzburg-Landau (GL) parameter of $κ= 0.70(5)$. The obtained $λ_L$ and $κ$ values, accurately quantified at the nanoscale, are smaller than values commonly used in applications and modeling, and indicate that clean niobium lies at the boundary between type-I and type-II superconductivity, supporting the contemporary view that its intrinsic state may be type-I.
title Niobium's intrinsic coherence length and penetration depth revisited using low-energy muon spin spectroscopy and secondary-ion mass spectrometry
topic Superconductivity
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2511.02913