Tunable Multistage Refrigeration via Geometrically Frustrated Triangular Lattice Antiferromagnet for Space Cooling

Fuente: arXiv
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Main Authors: Wang, Jianqiao, Fang, Chushu, Qiu, Zhibin, Zhao, Yang, Xiao, Quan, Sun, Xiying, Li, Zhaoyi, Li, Laifeng, Zhou, Yuan, Pan, Changzhao, Guo, Shu
Format: Preprint
Published: 2025
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author Wang, Jianqiao
Fang, Chushu
Qiu, Zhibin
Zhao, Yang
Xiao, Quan
Sun, Xiying
Li, Zhaoyi
Li, Laifeng
Zhou, Yuan
Pan, Changzhao
Guo, Shu
author_facet Wang, Jianqiao
Fang, Chushu
Qiu, Zhibin
Zhao, Yang
Xiao, Quan
Sun, Xiying
Li, Zhaoyi
Li, Laifeng
Zhou, Yuan
Pan, Changzhao
Guo, Shu
contents Low-temperature refrigeration technology constitutes a crucial component in space exploration. The small-scale, low-vibration Stirling-type pulse tube refrigerators hold significant application potential for space cooling. However, the efficient operation of current Stirling-type pulse tube cryocoolers in space cooling applications remains challenging due to the rapid decay of the heat capacity of regenerative materials below 10 K. This study adopts a novel material strategy: using a novel high-spin S = 7/2 magnetic regenerative material, Gd2O2Se, we construct a multistage tunable regenerative material structure to achieve an efficient cooling approach to the liquid helium temperature range. Under substantial geometric frustration from a double-layered triangular lattice, it exhibits two-step specific heat transition peaks at 6.22 K and 2.11 K, respectively. Its ultrahigh specific heat and broad two-step transition temperature range effectively bridge the gap between commercially used high-heat-capacity materials. Experimental verification shows that when Gd2O2Se is combined with Er3Ni and HoCu2 in the Stirling-type pulse tube cryocooler, the cooling efficiency of the pulse tube increases by 66.5 % at 7 K, and the minimum achievable temperature reaches 5.85 K. These results indicate that Gd2O2Se is an ideal magnetic regenerative material for space cooling
format Preprint
id arxiv_https___arxiv_org_abs_2511_03254
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Tunable Multistage Refrigeration via Geometrically Frustrated Triangular Lattice Antiferromagnet for Space Cooling
Wang, Jianqiao
Fang, Chushu
Qiu, Zhibin
Zhao, Yang
Xiao, Quan
Sun, Xiying
Li, Zhaoyi
Li, Laifeng
Zhou, Yuan
Pan, Changzhao
Guo, Shu
Materials Science
Low-temperature refrigeration technology constitutes a crucial component in space exploration. The small-scale, low-vibration Stirling-type pulse tube refrigerators hold significant application potential for space cooling. However, the efficient operation of current Stirling-type pulse tube cryocoolers in space cooling applications remains challenging due to the rapid decay of the heat capacity of regenerative materials below 10 K. This study adopts a novel material strategy: using a novel high-spin S = 7/2 magnetic regenerative material, Gd2O2Se, we construct a multistage tunable regenerative material structure to achieve an efficient cooling approach to the liquid helium temperature range. Under substantial geometric frustration from a double-layered triangular lattice, it exhibits two-step specific heat transition peaks at 6.22 K and 2.11 K, respectively. Its ultrahigh specific heat and broad two-step transition temperature range effectively bridge the gap between commercially used high-heat-capacity materials. Experimental verification shows that when Gd2O2Se is combined with Er3Ni and HoCu2 in the Stirling-type pulse tube cryocooler, the cooling efficiency of the pulse tube increases by 66.5 % at 7 K, and the minimum achievable temperature reaches 5.85 K. These results indicate that Gd2O2Se is an ideal magnetic regenerative material for space cooling
title Tunable Multistage Refrigeration via Geometrically Frustrated Triangular Lattice Antiferromagnet for Space Cooling
topic Materials Science
url https://arxiv.org/abs/2511.03254