Effects of crystal field and momentum-based frustrated exchange interactions on multiorbital square skyrmion lattice
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| Format: | Preprint |
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2025
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| author | Zha, Yan S. Hayami, Satoru |
| author_facet | Zha, Yan S. Hayami, Satoru |
| contents | Motivated by recent theoretical predictions of a square-shaped skyrmion lattice (S-SkL) in centrosymmetric tetragonal Ce-based magnets [Yan Zha and Satoru Hayami, Phys. Rev. B 111, 165155 (2025)], we perform a comprehensive theoretical investigation into the role of multiorbital effects and momentum-based frustrated exchange interactions in stabilizing such topologically nontrivial magnetic textures. By employing self-consistent mean-field calculations over a broad range of model parameters, we demonstrate that the cooperative interplay among interorbital coupling, frustrated exchange interactions at higher-harmonic wave vectors, and crystal-field-induced anisotropy is crucial for the stabilization of the S-SkL. Furthermore, the competition between the easy-plane intraorbital anisotropy and the easy-axis interorbital anisotropy leads to a significant enhancement of the S-SkL stability region. We also identify a rich variety of multi-$Q$ states, including a topologically nontrivial S-SkL state with a slight breaking of fourfold rotational symmetry (S-SkL$'$), magnetic bubble lattices (MBLs), and double-$Q$ phases with a local/net scalar chirality. Our findings elucidate the microscopic mechanism responsible for the emergence of S-SkLs in prototypical Ce-based magnets and provide a route toward realizing skyrmion lattices in a broader class of $f$-electron materials beyond conventional Gd- and Eu-based systems lacking orbital angular momentum. |
| format | Preprint |
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arxiv_https___arxiv_org_abs_2511_05896 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Effects of crystal field and momentum-based frustrated exchange interactions on multiorbital square skyrmion lattice Zha, Yan S. Hayami, Satoru Strongly Correlated Electrons Materials Science Motivated by recent theoretical predictions of a square-shaped skyrmion lattice (S-SkL) in centrosymmetric tetragonal Ce-based magnets [Yan Zha and Satoru Hayami, Phys. Rev. B 111, 165155 (2025)], we perform a comprehensive theoretical investigation into the role of multiorbital effects and momentum-based frustrated exchange interactions in stabilizing such topologically nontrivial magnetic textures. By employing self-consistent mean-field calculations over a broad range of model parameters, we demonstrate that the cooperative interplay among interorbital coupling, frustrated exchange interactions at higher-harmonic wave vectors, and crystal-field-induced anisotropy is crucial for the stabilization of the S-SkL. Furthermore, the competition between the easy-plane intraorbital anisotropy and the easy-axis interorbital anisotropy leads to a significant enhancement of the S-SkL stability region. We also identify a rich variety of multi-$Q$ states, including a topologically nontrivial S-SkL state with a slight breaking of fourfold rotational symmetry (S-SkL$'$), magnetic bubble lattices (MBLs), and double-$Q$ phases with a local/net scalar chirality. Our findings elucidate the microscopic mechanism responsible for the emergence of S-SkLs in prototypical Ce-based magnets and provide a route toward realizing skyrmion lattices in a broader class of $f$-electron materials beyond conventional Gd- and Eu-based systems lacking orbital angular momentum. |
| title | Effects of crystal field and momentum-based frustrated exchange interactions on multiorbital square skyrmion lattice |
| topic | Strongly Correlated Electrons Materials Science |
| url | https://arxiv.org/abs/2511.05896 |