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Main Authors: Seyler, Kyle L., Zhang, Hantao, Van Beveren, Daniel, Rotundu, Costel R., Lee, Young S., Cheng, Ran, Hsieh, David
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2511.07531
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author Seyler, Kyle L.
Zhang, Hantao
Van Beveren, Daniel
Rotundu, Costel R.
Lee, Young S.
Cheng, Ran
Hsieh, David
author_facet Seyler, Kyle L.
Zhang, Hantao
Van Beveren, Daniel
Rotundu, Costel R.
Lee, Young S.
Cheng, Ran
Hsieh, David
contents The ability to rapidly manipulate domain walls (DWs) in magnetic materials is key to developing novel high-speed spintronic memory and computing devices. Antiferromagnetic (AFM) materials present a particularly promising platform due to their robustness against stray fields and their potential for exceptional DW velocities. Among various proposed driving mechanisms, coherent spin waves could potentially propel AFM DWs to the magnon group velocity while minimizing dissipation from Joule heating. However, experimental realization has remained elusive due to the dual challenges of generating coherent AFM spin waves near isolated mobile AFM DWs and simultaneously measuring high-speed DW dynamics. Here we experimentally realize an approach where ultrafast laser pulses generate coherent spin waves that drive AFM DWs and develop a technique to directly map the spatiotemporal DW dynamics. Using the room-temperature AFM insulator Sr$_2$Cu$_3$O$_4$Cl$_2$, we observe AFM DW motion with record-high velocities up to ~50 km/s. Remarkably, the direction of DW propagation is controllable through both the pump laser helicity and the sign of the DW winding number. This bidirectional control can be theoretically explained, and numerically reproduced, by the DW dynamics induced by coherent spin waves of the in-plane magnon mode - a phenomenon unique to magnets with an easy-plane anisotropy. Our work uncovers a novel DW propulsion mechanism that is generalizable to a wide range of AFM materials, unlocking new opportunities for ultrafast coherent AFM spintronics.
format Preprint
id arxiv_https___arxiv_org_abs_2511_07531
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle High-speed antiferromagnetic domain walls driven by coherent spin waves
Seyler, Kyle L.
Zhang, Hantao
Van Beveren, Daniel
Rotundu, Costel R.
Lee, Young S.
Cheng, Ran
Hsieh, David
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
The ability to rapidly manipulate domain walls (DWs) in magnetic materials is key to developing novel high-speed spintronic memory and computing devices. Antiferromagnetic (AFM) materials present a particularly promising platform due to their robustness against stray fields and their potential for exceptional DW velocities. Among various proposed driving mechanisms, coherent spin waves could potentially propel AFM DWs to the magnon group velocity while minimizing dissipation from Joule heating. However, experimental realization has remained elusive due to the dual challenges of generating coherent AFM spin waves near isolated mobile AFM DWs and simultaneously measuring high-speed DW dynamics. Here we experimentally realize an approach where ultrafast laser pulses generate coherent spin waves that drive AFM DWs and develop a technique to directly map the spatiotemporal DW dynamics. Using the room-temperature AFM insulator Sr$_2$Cu$_3$O$_4$Cl$_2$, we observe AFM DW motion with record-high velocities up to ~50 km/s. Remarkably, the direction of DW propagation is controllable through both the pump laser helicity and the sign of the DW winding number. This bidirectional control can be theoretically explained, and numerically reproduced, by the DW dynamics induced by coherent spin waves of the in-plane magnon mode - a phenomenon unique to magnets with an easy-plane anisotropy. Our work uncovers a novel DW propulsion mechanism that is generalizable to a wide range of AFM materials, unlocking new opportunities for ultrafast coherent AFM spintronics.
title High-speed antiferromagnetic domain walls driven by coherent spin waves
topic Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
url https://arxiv.org/abs/2511.07531