Excitonic shift current induced broadband THz pulse emission efficiency of layered MoS2 crystals
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arXiv
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| Natura: | Preprint |
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2025
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| _version_ | 1866908916613382144 |
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| author | Dhakar, Neetesh Kumar, Sunil |
| author_facet | Dhakar, Neetesh Kumar, Sunil |
| contents | Following the ultrafast photoexcitation of a semiconductor, it embodies competing dynamics among photocarriers, many-body transient states of highly energetic excitons, and electron-hole liquid. Here, we show that femtosecond optical pulse excitation induces transient excitonic shift current contributing to stronger THz emission from a single crystalline bulk MoS2 at low temperatures. The control of dominating excitonic shift current is elucidated from excitation density dependent experiments at varying temperatures. A strong decrease in the excitonic contribution beyond a critical fluence of 150microJ/cm^2 is observed at a very low temperature of 20K. This behavior suggests the formation of a new quantum condensate, i.e., the electron-hole liquid, in the regime when the exciton density is overwhelmingly large that the average spacing between exciton pairs is comparable to the exciton radius. Furthermore, the exciton density dependent THz emission at varying temperatures is consistent with the Varshni model and the crystal Debye temperature of 260K. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2511_08166 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Excitonic shift current induced broadband THz pulse emission efficiency of layered MoS2 crystals Dhakar, Neetesh Kumar, Sunil Materials Science Optics Following the ultrafast photoexcitation of a semiconductor, it embodies competing dynamics among photocarriers, many-body transient states of highly energetic excitons, and electron-hole liquid. Here, we show that femtosecond optical pulse excitation induces transient excitonic shift current contributing to stronger THz emission from a single crystalline bulk MoS2 at low temperatures. The control of dominating excitonic shift current is elucidated from excitation density dependent experiments at varying temperatures. A strong decrease in the excitonic contribution beyond a critical fluence of 150microJ/cm^2 is observed at a very low temperature of 20K. This behavior suggests the formation of a new quantum condensate, i.e., the electron-hole liquid, in the regime when the exciton density is overwhelmingly large that the average spacing between exciton pairs is comparable to the exciton radius. Furthermore, the exciton density dependent THz emission at varying temperatures is consistent with the Varshni model and the crystal Debye temperature of 260K. |
| title | Excitonic shift current induced broadband THz pulse emission efficiency of layered MoS2 crystals |
| topic | Materials Science Optics |
| url | https://arxiv.org/abs/2511.08166 |