Cryogenic source of atomic tritium for neutrino-mass measurements and precision spectroscopy

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Main Authors: Semakin, Aleksei, Ahokas, Janne, Kiilerich, Tom, Vasiliev, Sergey, Nez, Francois, Yzombard, Pauline, Nesvizhevsky, Valery, Widmann, Eberhard, Crivelli, Paolo, Rodenbeck, Caroline, Röllig, Marco, Schlösser, Magnus
Format: Preprint
Published: 2025
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author Semakin, Aleksei
Ahokas, Janne
Kiilerich, Tom
Vasiliev, Sergey
Nez, Francois
Yzombard, Pauline
Nesvizhevsky, Valery
Widmann, Eberhard
Crivelli, Paolo
Rodenbeck, Caroline
Röllig, Marco
Schlösser, Magnus
author_facet Semakin, Aleksei
Ahokas, Janne
Kiilerich, Tom
Vasiliev, Sergey
Nez, Francois
Yzombard, Pauline
Nesvizhevsky, Valery
Widmann, Eberhard
Crivelli, Paolo
Rodenbeck, Caroline
Röllig, Marco
Schlösser, Magnus
contents We propose a concept for a cryogenic source of atomic tritium at sub-Kelvin temperatures and energies suitable for magnetic trapping. The source is based on the dissociation of solid molecular T2 films below 1 K by electrons from a pulsed RF discharge, a technique recently demonstrated for atomic hydrogen, combined with buffer-gas cooling and magnetic confinement. We analyze the key processes limiting the source performance, adsorption, spin exchange and recombination, and show that atomic tritium fluxes exceeding 1e15 1/s at kinetic energies of 100 mK can be achieved at the entrance to the magnetic trap. Such a source would enable Doppler-free two-photon 1S-2S spectroscopy in atomic tritium for high-precision measurements of the triton charge radius, providing a crucial benchmark for bound-state QED and improving the comparison between electronic, muonic, and scattering determinations of nuclear sizes in light systems. Beyond spectroscopy, an atomic tritium source avoids molecular final state broadening in the beta decay and is therefore necessary for next generation neutrino mass measurements; combined with detector technologies such as sub-eV resolution quantum sensors or cyclotron radiation emission spectroscopy, it enables an order of magnitude improvement compared to the current best experimental limit. Additionally, the source can be used to generate a beam of low field seeking deuterium atoms for loading magnetic traps, an important benchmark before trapping tritium atoms, which is useful for precision spectroscopy.
format Preprint
id arxiv_https___arxiv_org_abs_2511_08313
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Cryogenic source of atomic tritium for neutrino-mass measurements and precision spectroscopy
Semakin, Aleksei
Ahokas, Janne
Kiilerich, Tom
Vasiliev, Sergey
Nez, Francois
Yzombard, Pauline
Nesvizhevsky, Valery
Widmann, Eberhard
Crivelli, Paolo
Rodenbeck, Caroline
Röllig, Marco
Schlösser, Magnus
Atomic Physics
Nuclear Experiment
Instrumentation and Detectors
Quantum Physics
We propose a concept for a cryogenic source of atomic tritium at sub-Kelvin temperatures and energies suitable for magnetic trapping. The source is based on the dissociation of solid molecular T2 films below 1 K by electrons from a pulsed RF discharge, a technique recently demonstrated for atomic hydrogen, combined with buffer-gas cooling and magnetic confinement. We analyze the key processes limiting the source performance, adsorption, spin exchange and recombination, and show that atomic tritium fluxes exceeding 1e15 1/s at kinetic energies of 100 mK can be achieved at the entrance to the magnetic trap. Such a source would enable Doppler-free two-photon 1S-2S spectroscopy in atomic tritium for high-precision measurements of the triton charge radius, providing a crucial benchmark for bound-state QED and improving the comparison between electronic, muonic, and scattering determinations of nuclear sizes in light systems. Beyond spectroscopy, an atomic tritium source avoids molecular final state broadening in the beta decay and is therefore necessary for next generation neutrino mass measurements; combined with detector technologies such as sub-eV resolution quantum sensors or cyclotron radiation emission spectroscopy, it enables an order of magnitude improvement compared to the current best experimental limit. Additionally, the source can be used to generate a beam of low field seeking deuterium atoms for loading magnetic traps, an important benchmark before trapping tritium atoms, which is useful for precision spectroscopy.
title Cryogenic source of atomic tritium for neutrino-mass measurements and precision spectroscopy
topic Atomic Physics
Nuclear Experiment
Instrumentation and Detectors
Quantum Physics
url https://arxiv.org/abs/2511.08313