Reference Quadrupole Moments of Transition Elements from Lamb Shifts in Muonic Atoms

Fuente: arXiv
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Main Authors: Rathi, S., von Schoeler, K., Indelicato, P., Ohayon, B.
Format: Preprint
Published: 2025
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author Rathi, S.
von Schoeler, K.
Indelicato, P.
Ohayon, B.
author_facet Rathi, S.
von Schoeler, K.
Indelicato, P.
Ohayon, B.
contents We present a novel method for accurately measuring the absolute electric quadrupole moments of light transition elements $(23 \leq Z \leq 30 )$. Our approach is based on performing precision muonic x-ray spectroscopy of the $2s-2p$ manifold, which is also referred to as the Lamb shift. These transitions are too weak to be detected with dispersive methods and too overlapping to be resolved by solid-state detectors. Here, we propose the use of cryogenic microcalorimeters, which possess high efficiency and excellent energy resolution in the relevant energy regime, coupled with state-of-the-art theoretical calculations. We demonstrate the feasibility of this approach by performing extensive calculations and realistic simulations. In this way, we establish that the uncertainty in the absolute moment, which is transferred to the quadrupole moments of all isotopes in the chain, could be reduced by up to an order of magnitude within a day of measurement. These precise reference quadrupole moments serve as valuable inputs for nuclear structure studies and for benchmarking state-of-the-art quantum chemistry calculations in open-shell elements.
format Preprint
id arxiv_https___arxiv_org_abs_2511_17546
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Reference Quadrupole Moments of Transition Elements from Lamb Shifts in Muonic Atoms
Rathi, S.
von Schoeler, K.
Indelicato, P.
Ohayon, B.
Atomic Physics
Nuclear Experiment
We present a novel method for accurately measuring the absolute electric quadrupole moments of light transition elements $(23 \leq Z \leq 30 )$. Our approach is based on performing precision muonic x-ray spectroscopy of the $2s-2p$ manifold, which is also referred to as the Lamb shift. These transitions are too weak to be detected with dispersive methods and too overlapping to be resolved by solid-state detectors. Here, we propose the use of cryogenic microcalorimeters, which possess high efficiency and excellent energy resolution in the relevant energy regime, coupled with state-of-the-art theoretical calculations. We demonstrate the feasibility of this approach by performing extensive calculations and realistic simulations. In this way, we establish that the uncertainty in the absolute moment, which is transferred to the quadrupole moments of all isotopes in the chain, could be reduced by up to an order of magnitude within a day of measurement. These precise reference quadrupole moments serve as valuable inputs for nuclear structure studies and for benchmarking state-of-the-art quantum chemistry calculations in open-shell elements.
title Reference Quadrupole Moments of Transition Elements from Lamb Shifts in Muonic Atoms
topic Atomic Physics
Nuclear Experiment
url https://arxiv.org/abs/2511.17546