High-Accuracy Material Classification via Reference-Free Terahertz Spectroscopy: Revisiting Spectral Referencing and Feature Selection
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arXiv
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| Format: | Preprint |
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2025
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| _version_ | 1866914362909786112 |
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| author | Kristensen, Mathias Hedegaard Cielecki, Paweł Piotr Skovsen, Esben |
| author_facet | Kristensen, Mathias Hedegaard Cielecki, Paweł Piotr Skovsen, Esben |
| contents | We investigate how feature selection algorithms can enable accurate, reference-free classification of materials using sparse-frequency terahertz (THz) reflection spectroscopy. Three classes of feature selection strategies are evaluated. Namely, the filter-based mRMR (minimum Redundancy Maximum Relevance), the embedded LASSO (Least Absolute Shrinkage and Selection Operator), and the wrapper-based SFS (Sequential Forward Selection) algorithms. Each strategy is assessed using the Linear Logistic Regression, Naïve Bayes, and Support Vector Machine classifiers. Our results show that high classification accuracy can be achieved using only a small subset of frequencies. Particularly, when non-referenced spectra are applied. Furthermore, we show that the SFS-selected features align with the materials' absorption bands, confirming that the discriminative power arises from genuine spectroscopic contrasts. These findings highlights that reducing spectral dimensionality through data-driven selection eliminates the need for broadband sources and reference measurements, enabling compact, application-specific THz sensors. This approach offers robust material identification in real-world scenarios such as security screening, non-destructive testing, and environmental monitoring. |
| format | Preprint |
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arxiv_https___arxiv_org_abs_2511_18572 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | High-Accuracy Material Classification via Reference-Free Terahertz Spectroscopy: Revisiting Spectral Referencing and Feature Selection Kristensen, Mathias Hedegaard Cielecki, Paweł Piotr Skovsen, Esben Applied Physics Data Analysis, Statistics and Probability Optics We investigate how feature selection algorithms can enable accurate, reference-free classification of materials using sparse-frequency terahertz (THz) reflection spectroscopy. Three classes of feature selection strategies are evaluated. Namely, the filter-based mRMR (minimum Redundancy Maximum Relevance), the embedded LASSO (Least Absolute Shrinkage and Selection Operator), and the wrapper-based SFS (Sequential Forward Selection) algorithms. Each strategy is assessed using the Linear Logistic Regression, Naïve Bayes, and Support Vector Machine classifiers. Our results show that high classification accuracy can be achieved using only a small subset of frequencies. Particularly, when non-referenced spectra are applied. Furthermore, we show that the SFS-selected features align with the materials' absorption bands, confirming that the discriminative power arises from genuine spectroscopic contrasts. These findings highlights that reducing spectral dimensionality through data-driven selection eliminates the need for broadband sources and reference measurements, enabling compact, application-specific THz sensors. This approach offers robust material identification in real-world scenarios such as security screening, non-destructive testing, and environmental monitoring. |
| title | High-Accuracy Material Classification via Reference-Free Terahertz Spectroscopy: Revisiting Spectral Referencing and Feature Selection |
| topic | Applied Physics Data Analysis, Statistics and Probability Optics |
| url | https://arxiv.org/abs/2511.18572 |