Light-induced photomechanical patterning of ferroelectric polarization
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arXiv
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| Main Authors: | , , , , , , , , , , , , |
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| Format: | Preprint |
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2025
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| _version_ | 1866915660700844032 |
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| author | Degezelle, Alban Strobelt, Jonas Loebner, Sarah Mebarki, Moussa Fusil, Stephane Garcia, Vincent Berini, Bruno Polewczyk, Vincent Dumont, Yves Matzen, Sylvia Lecoeur, Philippe Santer, Svetlana Maroutian, Thomas |
| author_facet | Degezelle, Alban Strobelt, Jonas Loebner, Sarah Mebarki, Moussa Fusil, Stephane Garcia, Vincent Berini, Bruno Polewczyk, Vincent Dumont, Yves Matzen, Sylvia Lecoeur, Philippe Santer, Svetlana Maroutian, Thomas |
| contents | Tailoring at will polar textures in ferroelectrics is critical for the development of nanoscale electronics and functional oxide technologies. Freestanding ferroelectric membranes have enabled studies of strain-induced polarization responses, but the control over membrane shape and local polarization typically remains limited to spontaneous buckling or uniaxial mechanical deformations. In this work, we employ a versatile photosensitive-polymer patterning approach to impose programmable bending strain profiles in ferroelectric membranes. Using BaTiO3 as a model system, we demonstrate deterministic 90° polarization rotation driven by engineered in-plane strain, and 180° polarization reversal arising from flexoelectric coupling through a controlled strain gradient. These results establish this programmable bending as a powerful approach to investigate strain-dependent domain structures, leverage flexoelectric effects, and engineer custom ferroelectric landscapes across a wide range of oxide membranes. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2511_19029 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Light-induced photomechanical patterning of ferroelectric polarization Degezelle, Alban Strobelt, Jonas Loebner, Sarah Mebarki, Moussa Fusil, Stephane Garcia, Vincent Berini, Bruno Polewczyk, Vincent Dumont, Yves Matzen, Sylvia Lecoeur, Philippe Santer, Svetlana Maroutian, Thomas Materials Science Tailoring at will polar textures in ferroelectrics is critical for the development of nanoscale electronics and functional oxide technologies. Freestanding ferroelectric membranes have enabled studies of strain-induced polarization responses, but the control over membrane shape and local polarization typically remains limited to spontaneous buckling or uniaxial mechanical deformations. In this work, we employ a versatile photosensitive-polymer patterning approach to impose programmable bending strain profiles in ferroelectric membranes. Using BaTiO3 as a model system, we demonstrate deterministic 90° polarization rotation driven by engineered in-plane strain, and 180° polarization reversal arising from flexoelectric coupling through a controlled strain gradient. These results establish this programmable bending as a powerful approach to investigate strain-dependent domain structures, leverage flexoelectric effects, and engineer custom ferroelectric landscapes across a wide range of oxide membranes. |
| title | Light-induced photomechanical patterning of ferroelectric polarization |
| topic | Materials Science |
| url | https://arxiv.org/abs/2511.19029 |