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Autores principales: Huhtasaari, Johanna, Palakulam, Joyal Jain, Salha, Awse, Hyldgaard, Per, Schröder, Elsebeth, Berntsen, Magnus Hårdensson, Tjernberg, Oscar, Shah, Manasi, Martinez-Duarte, Rodrigo, He, Hans, Hofmann, Johannes, Bauch, Thilo, Shetty, Naveen, Lara-Avila, Samuel
Formato: Preprint
Publicado: 2025
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Acceso en línea:https://arxiv.org/abs/2512.00394
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author Huhtasaari, Johanna
Palakulam, Joyal Jain
Salha, Awse
Hyldgaard, Per
Schröder, Elsebeth
Berntsen, Magnus Hårdensson
Tjernberg, Oscar
Shah, Manasi
Martinez-Duarte, Rodrigo
He, Hans
Hofmann, Johannes
Bauch, Thilo
Shetty, Naveen
Lara-Avila, Samuel
author_facet Huhtasaari, Johanna
Palakulam, Joyal Jain
Salha, Awse
Hyldgaard, Per
Schröder, Elsebeth
Berntsen, Magnus Hårdensson
Tjernberg, Oscar
Shah, Manasi
Martinez-Duarte, Rodrigo
He, Hans
Hofmann, Johannes
Bauch, Thilo
Shetty, Naveen
Lara-Avila, Samuel
contents Producing large-area single-crystalline graphene is key to realizing its full potential in advanced applications, including twistronics. Yet, controlling graphene growth kinetics to avoid grain boundaries or multilayer growth remains challenging. Here, we demonstrate single-crystalline graphene free from multilayer domains via one-step delamination of epitaxial graphene from silicon carbide (SiC). This is enabled by a specific surface reconstruction of 4H-SiC(0001) achieved in our growth conditions. High crystalline quality is confirmed by the observation of the half-integer quantum Hall effect -- the hallmark of monolayer graphene -- in near cm-sized crystals. The scalability of our process, explored with 4''-wafers, represents an advance toward large-scale integration of high-performance graphene applications.
format Preprint
id arxiv_https___arxiv_org_abs_2512_00394
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Wafer-Scale Single-Crystalline Monolayer Graphene
Huhtasaari, Johanna
Palakulam, Joyal Jain
Salha, Awse
Hyldgaard, Per
Schröder, Elsebeth
Berntsen, Magnus Hårdensson
Tjernberg, Oscar
Shah, Manasi
Martinez-Duarte, Rodrigo
He, Hans
Hofmann, Johannes
Bauch, Thilo
Shetty, Naveen
Lara-Avila, Samuel
Mesoscale and Nanoscale Physics
Producing large-area single-crystalline graphene is key to realizing its full potential in advanced applications, including twistronics. Yet, controlling graphene growth kinetics to avoid grain boundaries or multilayer growth remains challenging. Here, we demonstrate single-crystalline graphene free from multilayer domains via one-step delamination of epitaxial graphene from silicon carbide (SiC). This is enabled by a specific surface reconstruction of 4H-SiC(0001) achieved in our growth conditions. High crystalline quality is confirmed by the observation of the half-integer quantum Hall effect -- the hallmark of monolayer graphene -- in near cm-sized crystals. The scalability of our process, explored with 4''-wafers, represents an advance toward large-scale integration of high-performance graphene applications.
title Wafer-Scale Single-Crystalline Monolayer Graphene
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2512.00394