Configurable antiferromagnetic domains and lateral exchange bias in atomically thin CrPS4

Fuente: arXiv
Guardado en:
Detalles Bibliográficos
Autores principales: Wang, Yu-Xuan, Graham, Thomas K. M., Rama-Eiroa, Ricardo, Islam, Md Ariful, Badarneh, Mohammad H., Gontijo, Rafael Nunes, Tiwari, Ganesh Prasad, Adhikari, Tibendra, Zhang, Xin-Yue, Watanabe, Kenji, Taniguchi, Takashi, Besson, Claire, Santos, Elton J. G., Lin, Zhong, Zhou, Brian B.
Formato: Preprint
Publicado: 2025
Materias:
Acceso en línea:
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
_version_ 1866918230414589952
author Wang, Yu-Xuan
Graham, Thomas K. M.
Rama-Eiroa, Ricardo
Islam, Md Ariful
Badarneh, Mohammad H.
Gontijo, Rafael Nunes
Tiwari, Ganesh Prasad
Adhikari, Tibendra
Zhang, Xin-Yue
Watanabe, Kenji
Taniguchi, Takashi
Besson, Claire
Santos, Elton J. G.
Lin, Zhong
Zhou, Brian B.
author_facet Wang, Yu-Xuan
Graham, Thomas K. M.
Rama-Eiroa, Ricardo
Islam, Md Ariful
Badarneh, Mohammad H.
Gontijo, Rafael Nunes
Tiwari, Ganesh Prasad
Adhikari, Tibendra
Zhang, Xin-Yue
Watanabe, Kenji
Taniguchi, Takashi
Besson, Claire
Santos, Elton J. G.
Lin, Zhong
Zhou, Brian B.
contents Interfacial exchange coupling between antiferromagnets (AFMs) and ferromagnets (FMs) crucially makes it possible to shift the FM hysteresis, known as exchange bias, and to switch AFM states. Two-dimensional magnets unlock opportunities to combine AFM and FM materials; however, the buried AFM-FM interfaces obtained by stacking remains challenging to understand. Here we demonstrate interfacial control via intralayer exchange coupling in the layered AFM CrPS$_4$, where connected even and odd layers realize pristine lateral interfaces between AFM-like and FM-like regions. We distinguish antiphase even-layer states by scanning nitrogen-vacancy centre (NV) magnetometry due to a weak surface magnetization. This surface magnetization enables control over the even-layer state, with different regions switching at distinct fields due to their own lateral couplings. We toggle three AFM domains adjacent to a FM-like region and demonstrate a tunable multilevel exchange bias. Our nanoscale visualization unveils the microscopic origins of exchange bias and advances single two-dimensional crystals for hybrid AFM-FM technologies.
format Preprint
id arxiv_https___arxiv_org_abs_2512_04055
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Configurable antiferromagnetic domains and lateral exchange bias in atomically thin CrPS4
Wang, Yu-Xuan
Graham, Thomas K. M.
Rama-Eiroa, Ricardo
Islam, Md Ariful
Badarneh, Mohammad H.
Gontijo, Rafael Nunes
Tiwari, Ganesh Prasad
Adhikari, Tibendra
Zhang, Xin-Yue
Watanabe, Kenji
Taniguchi, Takashi
Besson, Claire
Santos, Elton J. G.
Lin, Zhong
Zhou, Brian B.
Mesoscale and Nanoscale Physics
Interfacial exchange coupling between antiferromagnets (AFMs) and ferromagnets (FMs) crucially makes it possible to shift the FM hysteresis, known as exchange bias, and to switch AFM states. Two-dimensional magnets unlock opportunities to combine AFM and FM materials; however, the buried AFM-FM interfaces obtained by stacking remains challenging to understand. Here we demonstrate interfacial control via intralayer exchange coupling in the layered AFM CrPS$_4$, where connected even and odd layers realize pristine lateral interfaces between AFM-like and FM-like regions. We distinguish antiphase even-layer states by scanning nitrogen-vacancy centre (NV) magnetometry due to a weak surface magnetization. This surface magnetization enables control over the even-layer state, with different regions switching at distinct fields due to their own lateral couplings. We toggle three AFM domains adjacent to a FM-like region and demonstrate a tunable multilevel exchange bias. Our nanoscale visualization unveils the microscopic origins of exchange bias and advances single two-dimensional crystals for hybrid AFM-FM technologies.
title Configurable antiferromagnetic domains and lateral exchange bias in atomically thin CrPS4
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2512.04055