Optical Readout of Reconfigurable Layered Magnetic Domain Structure in CrSBr

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Auteurs principaux: Łopion, Aleksandra, Piel, Pierre-Maurice, Kliewer, Thomas, Terbeck, Manuel, Larusch, Jan-Hendrik, Henz, Jakob, Heißenbüttel, Marie-Christin, Mosina, Kseniia, Deilmann, Thorsten, Rohlfing, Michael, Sofer, Zdenek, Wurstbauer, Ursula
Format: Preprint
Publié: 2025
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author Łopion, Aleksandra
Piel, Pierre-Maurice
Kliewer, Thomas
Terbeck, Manuel
Larusch, Jan-Hendrik
Henz, Jakob
Heißenbüttel, Marie-Christin
Mosina, Kseniia
Deilmann, Thorsten
Rohlfing, Michael
Sofer, Zdenek
Wurstbauer, Ursula
author_facet Łopion, Aleksandra
Piel, Pierre-Maurice
Kliewer, Thomas
Terbeck, Manuel
Larusch, Jan-Hendrik
Henz, Jakob
Heißenbüttel, Marie-Christin
Mosina, Kseniia
Deilmann, Thorsten
Rohlfing, Michael
Sofer, Zdenek
Wurstbauer, Ursula
contents The van der Waals magnetic semiconductor CrSBr combines multistable magnetic order with strong light--matter coupling, enabling optical access to a rich and reconfigurable layered magnetic domain structure. A purely optical, non-destructive, and non-contact readout of layered magnetic configurations is realized here by magneto-reflectance measurements and interpreted using an optical multilayer model. The magnetic state is tunable by applied magnetic fields and by interfacing CrSBr with the antiferromagnet MnPS$_3$. Applying an external magnetic field along the easy axis drives the hysteretic antiferromagnetic--to--ferromagnetic transition, which is not universally binary but instead develops through a cascade of intermediate magnetic configurations whose multiplicity and stability scale systematically with layer thickness and can be tailored by magnetic interfaces. The intertwined optical and magnetic properties of CrSBr provide a readout mechanism for information encoded in and processed through its magnetic configuration that is compatible with modern on- and off-chip photonic and electronic technologies. These properties identify CrSBr as a promising platform for intelligent matter and for spin-optoelectronics, in particular for neuromorphic architectures that can learn and evolve in response to changing environments.
format Preprint
id arxiv_https___arxiv_org_abs_2512_04887
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Optical Readout of Reconfigurable Layered Magnetic Domain Structure in CrSBr
Łopion, Aleksandra
Piel, Pierre-Maurice
Kliewer, Thomas
Terbeck, Manuel
Larusch, Jan-Hendrik
Henz, Jakob
Heißenbüttel, Marie-Christin
Mosina, Kseniia
Deilmann, Thorsten
Rohlfing, Michael
Sofer, Zdenek
Wurstbauer, Ursula
Mesoscale and Nanoscale Physics
The van der Waals magnetic semiconductor CrSBr combines multistable magnetic order with strong light--matter coupling, enabling optical access to a rich and reconfigurable layered magnetic domain structure. A purely optical, non-destructive, and non-contact readout of layered magnetic configurations is realized here by magneto-reflectance measurements and interpreted using an optical multilayer model. The magnetic state is tunable by applied magnetic fields and by interfacing CrSBr with the antiferromagnet MnPS$_3$. Applying an external magnetic field along the easy axis drives the hysteretic antiferromagnetic--to--ferromagnetic transition, which is not universally binary but instead develops through a cascade of intermediate magnetic configurations whose multiplicity and stability scale systematically with layer thickness and can be tailored by magnetic interfaces. The intertwined optical and magnetic properties of CrSBr provide a readout mechanism for information encoded in and processed through its magnetic configuration that is compatible with modern on- and off-chip photonic and electronic technologies. These properties identify CrSBr as a promising platform for intelligent matter and for spin-optoelectronics, in particular for neuromorphic architectures that can learn and evolve in response to changing environments.
title Optical Readout of Reconfigurable Layered Magnetic Domain Structure in CrSBr
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2512.04887