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| Main Authors: | , , , |
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| Format: | Preprint |
| Published: |
2025
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| Subjects: | |
| Online Access: | https://arxiv.org/abs/2512.06599 |
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| _version_ | 1866914187273306112 |
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| author | Aliyev, Emin Mobaraki, Arash Sevinçli, Hâldun Jahangirov, Seymur |
| author_facet | Aliyev, Emin Mobaraki, Arash Sevinçli, Hâldun Jahangirov, Seymur |
| contents | Two-dimensional (2D) quartic dispersion materials are known to develop magnetization upon doping. Here we conduct a systematic investigation of magnetization in hole-doped quartic dispersion materials (GaS, InSe, TiO$_{2}$), focusing on the effects of structural confinement from 2D monolayers to quasi-one-dimensional nanoribbons (NRs). Upon hole doping, these NRs develop itinerant magnetization across a broad range of carrier densities and display half-metallic behavior. The spin-polarization energies ($E_{sp}$) of these NRs enhance remarkably relative to their 2D counterparts, with maximum increase being in the case of TiO$_{2}$ from 31 to 103 meV/carrier. The $E_{sp}$ strongly depends on the degree of localization of the magnetic moments along the width of NRs, which is determined by edge passivation and ribbon width. Strong deformation of the topmost valence bands at higher dopings indicates deviation from the Stoner mechanism. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2512_06599 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Doping induced magnetism and half-metallicity in nanoribbons of quartic dispersion materials Aliyev, Emin Mobaraki, Arash Sevinçli, Hâldun Jahangirov, Seymur Materials Science Mesoscale and Nanoscale Physics Two-dimensional (2D) quartic dispersion materials are known to develop magnetization upon doping. Here we conduct a systematic investigation of magnetization in hole-doped quartic dispersion materials (GaS, InSe, TiO$_{2}$), focusing on the effects of structural confinement from 2D monolayers to quasi-one-dimensional nanoribbons (NRs). Upon hole doping, these NRs develop itinerant magnetization across a broad range of carrier densities and display half-metallic behavior. The spin-polarization energies ($E_{sp}$) of these NRs enhance remarkably relative to their 2D counterparts, with maximum increase being in the case of TiO$_{2}$ from 31 to 103 meV/carrier. The $E_{sp}$ strongly depends on the degree of localization of the magnetic moments along the width of NRs, which is determined by edge passivation and ribbon width. Strong deformation of the topmost valence bands at higher dopings indicates deviation from the Stoner mechanism. |
| title | Doping induced magnetism and half-metallicity in nanoribbons of quartic dispersion materials |
| topic | Materials Science Mesoscale and Nanoscale Physics |
| url | https://arxiv.org/abs/2512.06599 |