High-harmonic generation driven by temporal-mode quantum states of light

Fuente: arXiv
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Main Authors: González-Monge, Juan M., Feist, Johannes
Format: Preprint
Published: 2025
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author González-Monge, Juan M.
Feist, Johannes
author_facet González-Monge, Juan M.
Feist, Johannes
contents We develop a theoretical framework for high-harmonic generation (HHG) driven by quantum states of light based on a temporal-mode expansion of the electromagnetic field. This approach extends previous single plane-wave mode treatments to realistic pulse configurations, resolving conceptual inconsistencies arising from non-normalizable infinite plane waves and establishing consistency between analytical and numerical methods. We derive a correction factor that quantifies deviations from the single-mode approximation and show that it remains below $10^{-4}$ for intensities typical of HHG ($\sim 10^{14}~$W/cm$^2$). This result confirms that free-space HHG driven by any quantum state of light is accurately described by averaging semi-classical calculations over the Husimi distribution, with no observable genuine quantum effects. The absence of such effects is attributed to the large photon numbers ($\sim 10^{11}$) required to reach HHG intensities in free space, which render quantum fluctuations negligible. We discuss nanophotonic environments with ultrasmall mode volumes as potential platforms where few-photon strong-field processes could exhibit genuine quantum signatures.
format Preprint
id arxiv_https___arxiv_org_abs_2512_06602
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle High-harmonic generation driven by temporal-mode quantum states of light
González-Monge, Juan M.
Feist, Johannes
Quantum Physics
Atomic Physics
We develop a theoretical framework for high-harmonic generation (HHG) driven by quantum states of light based on a temporal-mode expansion of the electromagnetic field. This approach extends previous single plane-wave mode treatments to realistic pulse configurations, resolving conceptual inconsistencies arising from non-normalizable infinite plane waves and establishing consistency between analytical and numerical methods. We derive a correction factor that quantifies deviations from the single-mode approximation and show that it remains below $10^{-4}$ for intensities typical of HHG ($\sim 10^{14}~$W/cm$^2$). This result confirms that free-space HHG driven by any quantum state of light is accurately described by averaging semi-classical calculations over the Husimi distribution, with no observable genuine quantum effects. The absence of such effects is attributed to the large photon numbers ($\sim 10^{11}$) required to reach HHG intensities in free space, which render quantum fluctuations negligible. We discuss nanophotonic environments with ultrasmall mode volumes as potential platforms where few-photon strong-field processes could exhibit genuine quantum signatures.
title High-harmonic generation driven by temporal-mode quantum states of light
topic Quantum Physics
Atomic Physics
url https://arxiv.org/abs/2512.06602