Atomic-scale probe of molecular magneto-electric coupling

Fuente: arXiv
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Autori principali: Amini, Mohammad, Yan, Linghao, Silveira, Orlando J., Fumega, Adolfo O., Vaňo, Viliam, Lado, Jose L., Kezilebieke, Shawulienu, Liljeroth, Peter, Drost, and Robert
Natura: Preprint
Pubblicazione: 2025
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author Amini, Mohammad
Yan, Linghao
Silveira, Orlando J.
Fumega, Adolfo O.
Vaňo, Viliam
Lado, Jose L.
Kezilebieke, Shawulienu
Liljeroth, Peter
Drost, and Robert
author_facet Amini, Mohammad
Yan, Linghao
Silveira, Orlando J.
Fumega, Adolfo O.
Vaňo, Viliam
Lado, Jose L.
Kezilebieke, Shawulienu
Liljeroth, Peter
Drost, and Robert
contents Van der Waals heterostructures are a core tool in quantum material design. The recent addition of monolayer ferroelectrics expands the possibilities of designer materials. Ferroelectric domains can be manipulated using electric fields, thus opening a route for external control over material properties. In this paper we explore the possibility of engineering magneto-electric coupling in ferroelectric heterostructures by studying the interface of bilayer SnTe with iron phthalocyanine molecules as a model system. The molecules act as sensor spins, allowing us to sample the magneto-electric coupling with nanometer precision through scanning tunneling microscopy. Our measurements uncover a structural, and therefore material-independent and intrinsic, mechanism to couple electric and magnetic degrees of freedom at the nanoscale.
format Preprint
id arxiv_https___arxiv_org_abs_2512_07489
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Atomic-scale probe of molecular magneto-electric coupling
Amini, Mohammad
Yan, Linghao
Silveira, Orlando J.
Fumega, Adolfo O.
Vaňo, Viliam
Lado, Jose L.
Kezilebieke, Shawulienu
Liljeroth, Peter
Drost, and Robert
Mesoscale and Nanoscale Physics
Van der Waals heterostructures are a core tool in quantum material design. The recent addition of monolayer ferroelectrics expands the possibilities of designer materials. Ferroelectric domains can be manipulated using electric fields, thus opening a route for external control over material properties. In this paper we explore the possibility of engineering magneto-electric coupling in ferroelectric heterostructures by studying the interface of bilayer SnTe with iron phthalocyanine molecules as a model system. The molecules act as sensor spins, allowing us to sample the magneto-electric coupling with nanometer precision through scanning tunneling microscopy. Our measurements uncover a structural, and therefore material-independent and intrinsic, mechanism to couple electric and magnetic degrees of freedom at the nanoscale.
title Atomic-scale probe of molecular magneto-electric coupling
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2512.07489