Magnetic properties of the Fe$_5$SiB$_2$-Fe$_5$PB$_2$ system

Fuente: arXiv
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Autori principali: Hedlund, Daniel, Cedervall, Johan, Edström, Alexander, Werwinski, Mirosław, Eriksson, Sofia Kontos Olle, Rusz, Ján, Svedlindh, Peter, Sahlberg, Martin, Gunnarsson, Klas
Natura: Preprint
Pubblicazione: 2025
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author Hedlund, Daniel
Cedervall, Johan
Edström, Alexander
Werwinski, Mirosław
Eriksson, Sofia Kontos Olle
Rusz, Ján
Svedlindh, Peter
Sahlberg, Martin
Gunnarsson, Klas
author_facet Hedlund, Daniel
Cedervall, Johan
Edström, Alexander
Werwinski, Mirosław
Eriksson, Sofia Kontos Olle
Rusz, Ján
Svedlindh, Peter
Sahlberg, Martin
Gunnarsson, Klas
contents The magnetic properties of the compound Fe$_5$Si$_{1-x}$P$_{x}$B$_2$ have been studied, with a focus on the Curie temperature $T_\textrm{C}$, saturation magnetization $M_\textrm{S}$, and magnetocrystalline anisotropy. Field and temperature dependent magnetization measurements were used to determine $T_\textrm{C}\left(x\right)$ and $M_\textrm{S}\left(x\right)$. The saturation magnetization at 10 K (300 K) is found to monotonically decrease from $1.11~\mathrm{MA/m}$ ($1.03~\mathrm{MA/m}$) to $0.97~\mathrm{MA/m}$ ($0.87~\mathrm{MA/m}$), as $x$ increases from zero to one. The Curie temperature is determined to be 810 K and 615 K in Fe$_5$SiB$_2$ and Fe$_5$PB$_2$, respectively. The highest $T_\textrm{C}$ is observed for $x=0.1$, while it decreases monotonically for larger $x$. The Curie temperatures have also been theoretically determined to be 700 K and 660 K for Fe$_5$SiB$_2$ and Fe$_5$PB$_2$, respectively, using a combination of density functional theory and Monte Carlo simulations. The magnitude of the effective magnetocrystalline anisotropy was extracted using the law of approach to saturation, revealing an increase with increasing phosphorus concentration. Low--field magnetization vs. temperature results for $x = 0, 0.1, 0.2$ indicate that there is a transition from easy--axis to easy--plane anisotropy with decreasing temperature.
format Preprint
id arxiv_https___arxiv_org_abs_2512_08043
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Magnetic properties of the Fe$_5$SiB$_2$-Fe$_5$PB$_2$ system
Hedlund, Daniel
Cedervall, Johan
Edström, Alexander
Werwinski, Mirosław
Eriksson, Sofia Kontos Olle
Rusz, Ján
Svedlindh, Peter
Sahlberg, Martin
Gunnarsson, Klas
Materials Science
The magnetic properties of the compound Fe$_5$Si$_{1-x}$P$_{x}$B$_2$ have been studied, with a focus on the Curie temperature $T_\textrm{C}$, saturation magnetization $M_\textrm{S}$, and magnetocrystalline anisotropy. Field and temperature dependent magnetization measurements were used to determine $T_\textrm{C}\left(x\right)$ and $M_\textrm{S}\left(x\right)$. The saturation magnetization at 10 K (300 K) is found to monotonically decrease from $1.11~\mathrm{MA/m}$ ($1.03~\mathrm{MA/m}$) to $0.97~\mathrm{MA/m}$ ($0.87~\mathrm{MA/m}$), as $x$ increases from zero to one. The Curie temperature is determined to be 810 K and 615 K in Fe$_5$SiB$_2$ and Fe$_5$PB$_2$, respectively. The highest $T_\textrm{C}$ is observed for $x=0.1$, while it decreases monotonically for larger $x$. The Curie temperatures have also been theoretically determined to be 700 K and 660 K for Fe$_5$SiB$_2$ and Fe$_5$PB$_2$, respectively, using a combination of density functional theory and Monte Carlo simulations. The magnitude of the effective magnetocrystalline anisotropy was extracted using the law of approach to saturation, revealing an increase with increasing phosphorus concentration. Low--field magnetization vs. temperature results for $x = 0, 0.1, 0.2$ indicate that there is a transition from easy--axis to easy--plane anisotropy with decreasing temperature.
title Magnetic properties of the Fe$_5$SiB$_2$-Fe$_5$PB$_2$ system
topic Materials Science
url https://arxiv.org/abs/2512.08043