Low-dimensionality-induced tunable ferromagnetism in SrRuO$_3$ ultrathin films
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arXiv
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| Autores principales: | , , , , , , , |
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| Formato: | Preprint |
| Publicado: |
2025
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| _version_ | 1866915702990962688 |
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| author | Kim, Jinyoung Kim, Minjae Kim, Donghan Hahn, Sungsoo Kim, Younsik Kim, Minsoo Sohn, Byungmin Kim, Changyoung |
| author_facet | Kim, Jinyoung Kim, Minjae Kim, Donghan Hahn, Sungsoo Kim, Younsik Kim, Minsoo Sohn, Byungmin Kim, Changyoung |
| contents | Quantum materials near electronic or magnetic phase boundaries exhibit enhanced tunability, as their emergent properties become highly sensitive to external perturbations. Here, we demonstrate precise control of ferromagnetism in a SrRuO$_3$ ultrathin film, where a high density of states (DOS), arising from low-dimensional quantum states, places the system at the crossover between a non-magnetic and bulk ferromagnetic state. Using spin- and angle-resolved photoemission spectroscopy (SRPES/ARPES), transport measurements, and theoretical calculations, we systematically tune the Fermi level via electron doping across the high-DOS point. We directly visualize the spin-split band structure and reveal its influence on both magnetic and transport properties. Our findings provide compelling evidence that magnetism can be engineered through DOS control at a phase crossover, establishing a pathway for the rational design of tunable quantum materials. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2512_09320 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Low-dimensionality-induced tunable ferromagnetism in SrRuO$_3$ ultrathin films Kim, Jinyoung Kim, Minjae Kim, Donghan Hahn, Sungsoo Kim, Younsik Kim, Minsoo Sohn, Byungmin Kim, Changyoung Strongly Correlated Electrons Materials Science Quantum materials near electronic or magnetic phase boundaries exhibit enhanced tunability, as their emergent properties become highly sensitive to external perturbations. Here, we demonstrate precise control of ferromagnetism in a SrRuO$_3$ ultrathin film, where a high density of states (DOS), arising from low-dimensional quantum states, places the system at the crossover between a non-magnetic and bulk ferromagnetic state. Using spin- and angle-resolved photoemission spectroscopy (SRPES/ARPES), transport measurements, and theoretical calculations, we systematically tune the Fermi level via electron doping across the high-DOS point. We directly visualize the spin-split band structure and reveal its influence on both magnetic and transport properties. Our findings provide compelling evidence that magnetism can be engineered through DOS control at a phase crossover, establishing a pathway for the rational design of tunable quantum materials. |
| title | Low-dimensionality-induced tunable ferromagnetism in SrRuO$_3$ ultrathin films |
| topic | Strongly Correlated Electrons Materials Science |
| url | https://arxiv.org/abs/2512.09320 |