Interplay between charge correlations and superconductivity across the superconducting domes of CsV$_{3}$Sb$_{5-x}$Sn$_x$

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Hauptverfasser: Salinas, Andrea N. Capa, Ortiz, Brenden R., Alvarado, Steven J. Gomez, Schwarz, Sarah, Pokharel, Ganesh, Buiarelli, Luca, Park, Hyeonseo Harry, Yuan, Shiyu, Yin, Roland, Sarker, Suchismita, Birol, Turan, Wilson, Stephen D.
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Veröffentlicht: 2025
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author Salinas, Andrea N. Capa
Ortiz, Brenden R.
Alvarado, Steven J. Gomez
Schwarz, Sarah
Pokharel, Ganesh
Buiarelli, Luca
Park, Hyeonseo Harry
Yuan, Shiyu
Yin, Roland
Sarker, Suchismita
Birol, Turan
Wilson, Stephen D.
author_facet Salinas, Andrea N. Capa
Ortiz, Brenden R.
Alvarado, Steven J. Gomez
Schwarz, Sarah
Pokharel, Ganesh
Buiarelli, Luca
Park, Hyeonseo Harry
Yuan, Shiyu
Yin, Roland
Sarker, Suchismita
Birol, Turan
Wilson, Stephen D.
contents The kagome metal CsV$_3$Sb$_5$ shows an unconventional interplay between charge density wave (CDW) order and superconductivity. Tuning the band filling is known to rapidly suppress long-range CDW order and drive the formation of two superconducting ``domes" upon increasing hole concentration. Here we determine the detailed evolution of charge correlations across this phase diagram and resolve their interplay with the superconducting state. Upon light hole-doping, the suppression of a metastable $2\times 2\times 4$ CDW state coincides with the suppression of superconducting fluctuations present in the parent CsV$_3$Sb$_5$ compound. Continued doping suppresses long-range $2\times 2\times 2$ CDW order, leaving remnant short-range, quasi-1D correlations that persist across the second superconducting dome. These higher temperature charge correlations are seemingly essential to the lower temperature superconducting state, as charge correlations vanish coincident with superconductivity as a function of hole-doping. A multidomain model of short-range V-V dimer formation within the kagome plane is proposed in the second superconducting dome, where rotational and translational symmetry remain locally broken even in the absence of long-range CDW order.
format Preprint
id arxiv_https___arxiv_org_abs_2512_11177
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Interplay between charge correlations and superconductivity across the superconducting domes of CsV$_{3}$Sb$_{5-x}$Sn$_x$
Salinas, Andrea N. Capa
Ortiz, Brenden R.
Alvarado, Steven J. Gomez
Schwarz, Sarah
Pokharel, Ganesh
Buiarelli, Luca
Park, Hyeonseo Harry
Yuan, Shiyu
Yin, Roland
Sarker, Suchismita
Birol, Turan
Wilson, Stephen D.
Superconductivity
Strongly Correlated Electrons
The kagome metal CsV$_3$Sb$_5$ shows an unconventional interplay between charge density wave (CDW) order and superconductivity. Tuning the band filling is known to rapidly suppress long-range CDW order and drive the formation of two superconducting ``domes" upon increasing hole concentration. Here we determine the detailed evolution of charge correlations across this phase diagram and resolve their interplay with the superconducting state. Upon light hole-doping, the suppression of a metastable $2\times 2\times 4$ CDW state coincides with the suppression of superconducting fluctuations present in the parent CsV$_3$Sb$_5$ compound. Continued doping suppresses long-range $2\times 2\times 2$ CDW order, leaving remnant short-range, quasi-1D correlations that persist across the second superconducting dome. These higher temperature charge correlations are seemingly essential to the lower temperature superconducting state, as charge correlations vanish coincident with superconductivity as a function of hole-doping. A multidomain model of short-range V-V dimer formation within the kagome plane is proposed in the second superconducting dome, where rotational and translational symmetry remain locally broken even in the absence of long-range CDW order.
title Interplay between charge correlations and superconductivity across the superconducting domes of CsV$_{3}$Sb$_{5-x}$Sn$_x$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2512.11177