Third Harmonic Generation in Transparent Longitudinal Epsilon-Near-Zero Multilayers

Fuente: arXiv
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Main Authors: Jaffray, Wallace, Stengel, Sven, de Ceglia, Domenico, Akozbek, Neset, Capolino, Filippo, Ferrera, Marcello, Scalora, Michael, Vincenti, Maria Antonietta
Format: Preprint
Published: 2025
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author Jaffray, Wallace
Stengel, Sven
de Ceglia, Domenico
Akozbek, Neset
Capolino, Filippo
Ferrera, Marcello
Scalora, Michael
Vincenti, Maria Antonietta
author_facet Jaffray, Wallace
Stengel, Sven
de Ceglia, Domenico
Akozbek, Neset
Capolino, Filippo
Ferrera, Marcello
Scalora, Michael
Vincenti, Maria Antonietta
contents Epsilon near zero (ENZ) materials can dramatically enhance local optical fields, enabling nonlinear interactions at relatively low intensities. Yet, near their plasma frequency, conventional isotropic ENZ media remain highly absorptive, limiting nonlinear operations that require good transparency. Longitudinal epsilon near zero metamaterials (LENZ), characterized by a vanishing permittivity along the optical axis provide an exceptional platform for field enhancement while mitigating absorption losses and impedance mismatch. We experimentally show that a Si and ITO multilayer engineered for a LENZ resonance in the near-infrared enables broadband, high pump transmission while still harnessing ENZ enhanced nonlinearity to generate a strong third harmonic signal. This demonstrates that efficient nonlinear processes can be driven without the high-loss conditions typical of isotropic ENZ media and regardless of intrinsic absorption at the harmonic frequency. The resulting third harmonic efficiency is comparable to isotropic ENZ films but without the absorption-induced heating constraints of ENZ operation. The high pump transmission enables transparent LENZ (TLENZ) stacks to be integrated into optical cavities, where resonant field buildup could amplify the nonlinear response without compromising thermal management. These results establish TLENZ multilayers as a robust, versatile platform for transparent, field enhanced nonlinear nanophotonics, combining strong light matter interaction with low-loss operation.
format Preprint
id arxiv_https___arxiv_org_abs_2512_13141
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Third Harmonic Generation in Transparent Longitudinal Epsilon-Near-Zero Multilayers
Jaffray, Wallace
Stengel, Sven
de Ceglia, Domenico
Akozbek, Neset
Capolino, Filippo
Ferrera, Marcello
Scalora, Michael
Vincenti, Maria Antonietta
Optics
78
J.2
Epsilon near zero (ENZ) materials can dramatically enhance local optical fields, enabling nonlinear interactions at relatively low intensities. Yet, near their plasma frequency, conventional isotropic ENZ media remain highly absorptive, limiting nonlinear operations that require good transparency. Longitudinal epsilon near zero metamaterials (LENZ), characterized by a vanishing permittivity along the optical axis provide an exceptional platform for field enhancement while mitigating absorption losses and impedance mismatch. We experimentally show that a Si and ITO multilayer engineered for a LENZ resonance in the near-infrared enables broadband, high pump transmission while still harnessing ENZ enhanced nonlinearity to generate a strong third harmonic signal. This demonstrates that efficient nonlinear processes can be driven without the high-loss conditions typical of isotropic ENZ media and regardless of intrinsic absorption at the harmonic frequency. The resulting third harmonic efficiency is comparable to isotropic ENZ films but without the absorption-induced heating constraints of ENZ operation. The high pump transmission enables transparent LENZ (TLENZ) stacks to be integrated into optical cavities, where resonant field buildup could amplify the nonlinear response without compromising thermal management. These results establish TLENZ multilayers as a robust, versatile platform for transparent, field enhanced nonlinear nanophotonics, combining strong light matter interaction with low-loss operation.
title Third Harmonic Generation in Transparent Longitudinal Epsilon-Near-Zero Multilayers
topic Optics
78
J.2
url https://arxiv.org/abs/2512.13141