Tuning Carrier Type and Density in Highly Conductive and Infrared-Transparent (Bi1-xSbx)2Te3 films

Fuente: arXiv
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Main Authors: Zeng, Xiangren, Zhang, Shenjin, Li, Zhiheng, Ma, Weiyue, Xie, Renjie, Cao, Yanwei, Liu, Fengguang, Zhang, Fengfeng, Zhao, Haichao, Yao, Xiong
Format: Preprint
Published: 2025
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author Zeng, Xiangren
Zhang, Shenjin
Li, Zhiheng
Ma, Weiyue
Xie, Renjie
Cao, Yanwei
Liu, Fengguang
Zhang, Fengfeng
Zhao, Haichao
Yao, Xiong
author_facet Zeng, Xiangren
Zhang, Shenjin
Li, Zhiheng
Ma, Weiyue
Xie, Renjie
Cao, Yanwei
Liu, Fengguang
Zhang, Fengfeng
Zhao, Haichao
Yao, Xiong
contents Infrared transparent conductors have long been sought due to their broad optoelectronic applications in the infrared wavelength range. However, the search for ideal materials has been limited by the inherent trade-off between electrical conductance and optical transmittance. Band engineering offers an effective approach to modulate carrier type and density, enabling concurrent tuning of both conductance and transmittance. In this work, we present a band engineering strategy that enables effective tuning of both infrared transmittance and electrical conductance in topological insulator (Bi1-xSbx)2Te3, bridging the gap and paving the way for applying topological insulators to infrared photoelectric devices. More importantly, with the combination of high carrier mobility and a large optical dielectric constant as suggested by previous report, Sb2Te3 achieves a high electrical conductance (~1000 S/cm) and outstanding infrared transmittance (92.3%) in the wavelength range of 8~13 um, demonstrating strong potential as an infrared transparent conductor. Our findings reveal that concurrent enhancement of both carrier mobility and optical dielectric constant is key to overcoming the conductance-transmittance trade-off. This work provides valuable insight for the exploration of high-performance infrared transparent conducting materials.
format Preprint
id arxiv_https___arxiv_org_abs_2512_16064
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Tuning Carrier Type and Density in Highly Conductive and Infrared-Transparent (Bi1-xSbx)2Te3 films
Zeng, Xiangren
Zhang, Shenjin
Li, Zhiheng
Ma, Weiyue
Xie, Renjie
Cao, Yanwei
Liu, Fengguang
Zhang, Fengfeng
Zhao, Haichao
Yao, Xiong
Materials Science
Mesoscale and Nanoscale Physics
Infrared transparent conductors have long been sought due to their broad optoelectronic applications in the infrared wavelength range. However, the search for ideal materials has been limited by the inherent trade-off between electrical conductance and optical transmittance. Band engineering offers an effective approach to modulate carrier type and density, enabling concurrent tuning of both conductance and transmittance. In this work, we present a band engineering strategy that enables effective tuning of both infrared transmittance and electrical conductance in topological insulator (Bi1-xSbx)2Te3, bridging the gap and paving the way for applying topological insulators to infrared photoelectric devices. More importantly, with the combination of high carrier mobility and a large optical dielectric constant as suggested by previous report, Sb2Te3 achieves a high electrical conductance (~1000 S/cm) and outstanding infrared transmittance (92.3%) in the wavelength range of 8~13 um, demonstrating strong potential as an infrared transparent conductor. Our findings reveal that concurrent enhancement of both carrier mobility and optical dielectric constant is key to overcoming the conductance-transmittance trade-off. This work provides valuable insight for the exploration of high-performance infrared transparent conducting materials.
title Tuning Carrier Type and Density in Highly Conductive and Infrared-Transparent (Bi1-xSbx)2Te3 films
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2512.16064