Picosecond localization dynamics following ultrafast nanoscale magnetic switching

Fuente: arXiv
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Autores principales: Metternich, Daniel, Schneider, Michael, Mercurio, Giuseppe, Hegstad, Torstein, Möller, Marcel, Battistelli, Riccardo, Klose, Christopher, Wittrock, Steffen, Patra, Manas R., Joy, Krishnanjana Puzhekadavil, Deinhart, Victor, Petz, Sascha, Prokes, Karel, Wintz, Sebastian, Weigand, Markus, Engel, Wolfgang-Dietrich, Sidiropoulos, Themistoklis, Will, Ingo, Eisebitt, Stefan, Carley, Robert E., Mercadier, Laurent, Schlappa, Justine, Teichmann, Martin, Scherz, Andreas, Zayko, Sergey, Sorokin, Boris V., Bagschik, Kai, Ropers, Claus, Mentink, Johan H., Pfau, Bastian, Büttner, Felix
Formato: Preprint
Publicado: 2025
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author Metternich, Daniel
Schneider, Michael
Mercurio, Giuseppe
Hegstad, Torstein
Möller, Marcel
Battistelli, Riccardo
Klose, Christopher
Wittrock, Steffen
Patra, Manas R.
Joy, Krishnanjana Puzhekadavil
Deinhart, Victor
Petz, Sascha
Prokes, Karel
Wintz, Sebastian
Weigand, Markus
Engel, Wolfgang-Dietrich
Sidiropoulos, Themistoklis
Will, Ingo
Eisebitt, Stefan
Carley, Robert E.
Mercadier, Laurent
Schlappa, Justine
Teichmann, Martin
Scherz, Andreas
Zayko, Sergey
Sorokin, Boris V.
Bagschik, Kai
Ropers, Claus
Mentink, Johan H.
Pfau, Bastian
Büttner, Felix
author_facet Metternich, Daniel
Schneider, Michael
Mercurio, Giuseppe
Hegstad, Torstein
Möller, Marcel
Battistelli, Riccardo
Klose, Christopher
Wittrock, Steffen
Patra, Manas R.
Joy, Krishnanjana Puzhekadavil
Deinhart, Victor
Petz, Sascha
Prokes, Karel
Wintz, Sebastian
Weigand, Markus
Engel, Wolfgang-Dietrich
Sidiropoulos, Themistoklis
Will, Ingo
Eisebitt, Stefan
Carley, Robert E.
Mercadier, Laurent
Schlappa, Justine
Teichmann, Martin
Scherz, Andreas
Zayko, Sergey
Sorokin, Boris V.
Bagschik, Kai
Ropers, Claus
Mentink, Johan H.
Pfau, Bastian
Büttner, Felix
contents Ultrashort laser pulses provide the fastest known way to switch magnetic order. Such excitation commonly creates nanometer-scale domains, even after homogeneous illumination when the position of nucleated domains is not externally defined. However, the physics of domain localization during such ultrafast phase transitions remains unresolved. Here, we use shot-resolved pump-probe resonant x-ray scattering together with a material featuring a periodically modulated magnetic anisotropy landscape to track, in real time, the laser-driven nucleation and localization of nanometer-scale spin textures. We find that nucleation and localization are two distinct processes. Nucleation occurs homogeneously via fluctuations at early times, whereas spatially periodic structures emerge only later and, under suitable conditions, localize in less than one nanosecond. Real-space simulations show that this localization is governed by strong lateral variations in spin-texture lifetimes. Our results demonstrate that ultrafast phase-transition dynamics fundamentally differ from conventional transitions, yet still can be controlled through moderate nanometer-scale tailoring of the energy landscape.
format Preprint
id arxiv_https___arxiv_org_abs_2512_17643
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Picosecond localization dynamics following ultrafast nanoscale magnetic switching
Metternich, Daniel
Schneider, Michael
Mercurio, Giuseppe
Hegstad, Torstein
Möller, Marcel
Battistelli, Riccardo
Klose, Christopher
Wittrock, Steffen
Patra, Manas R.
Joy, Krishnanjana Puzhekadavil
Deinhart, Victor
Petz, Sascha
Prokes, Karel
Wintz, Sebastian
Weigand, Markus
Engel, Wolfgang-Dietrich
Sidiropoulos, Themistoklis
Will, Ingo
Eisebitt, Stefan
Carley, Robert E.
Mercadier, Laurent
Schlappa, Justine
Teichmann, Martin
Scherz, Andreas
Zayko, Sergey
Sorokin, Boris V.
Bagschik, Kai
Ropers, Claus
Mentink, Johan H.
Pfau, Bastian
Büttner, Felix
Mesoscale and Nanoscale Physics
Ultrashort laser pulses provide the fastest known way to switch magnetic order. Such excitation commonly creates nanometer-scale domains, even after homogeneous illumination when the position of nucleated domains is not externally defined. However, the physics of domain localization during such ultrafast phase transitions remains unresolved. Here, we use shot-resolved pump-probe resonant x-ray scattering together with a material featuring a periodically modulated magnetic anisotropy landscape to track, in real time, the laser-driven nucleation and localization of nanometer-scale spin textures. We find that nucleation and localization are two distinct processes. Nucleation occurs homogeneously via fluctuations at early times, whereas spatially periodic structures emerge only later and, under suitable conditions, localize in less than one nanosecond. Real-space simulations show that this localization is governed by strong lateral variations in spin-texture lifetimes. Our results demonstrate that ultrafast phase-transition dynamics fundamentally differ from conventional transitions, yet still can be controlled through moderate nanometer-scale tailoring of the energy landscape.
title Picosecond localization dynamics following ultrafast nanoscale magnetic switching
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2512.17643