Clever Hans in Chemistry: Chemist Style Signals Confound Activity Prediction on Public Benchmarks

Fuente: arXiv
Saved in:
Bibliographic Details
Main Authors: Blevins, Andrew D., Quigley, Ian K.
Format: Preprint
Published: 2025
Subjects:
Online Access:
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866917168758652928
author Blevins, Andrew D.
Quigley, Ian K.
author_facet Blevins, Andrew D.
Quigley, Ian K.
contents Can machine learning models identify which chemist made a molecule from structure alone? If so, models trained on literature data may exploit chemist intent rather than learning causal structure-activity relationships. We test this by linking CHEMBL assays to publication authors and training a 1,815-class classifier to predict authors from molecular fingerprints, achieving 60% top-5 accuracy under scaffold-based splitting. We then train an activity model that receives only a protein identifier and an author-probability vector derived from structure, with no direct access to molecular descriptors. This author-only model achieves predictive power comparable to a simple baseline that has access to structure. This reveals a "Clever Hans" failure mode: models can predict bioactivity largely by inferring chemist goals and favorite targets without requiring a lab-independent understanding of chemistry. We analyze the sources of this leakage, propose author-disjoint splits, and recommend dataset practices to decouple chemist intent from biological outcomes.
format Preprint
id arxiv_https___arxiv_org_abs_2512_20924
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Clever Hans in Chemistry: Chemist Style Signals Confound Activity Prediction on Public Benchmarks
Blevins, Andrew D.
Quigley, Ian K.
Biomolecules
Machine Learning
Chemical Physics
Can machine learning models identify which chemist made a molecule from structure alone? If so, models trained on literature data may exploit chemist intent rather than learning causal structure-activity relationships. We test this by linking CHEMBL assays to publication authors and training a 1,815-class classifier to predict authors from molecular fingerprints, achieving 60% top-5 accuracy under scaffold-based splitting. We then train an activity model that receives only a protein identifier and an author-probability vector derived from structure, with no direct access to molecular descriptors. This author-only model achieves predictive power comparable to a simple baseline that has access to structure. This reveals a "Clever Hans" failure mode: models can predict bioactivity largely by inferring chemist goals and favorite targets without requiring a lab-independent understanding of chemistry. We analyze the sources of this leakage, propose author-disjoint splits, and recommend dataset practices to decouple chemist intent from biological outcomes.
title Clever Hans in Chemistry: Chemist Style Signals Confound Activity Prediction on Public Benchmarks
topic Biomolecules
Machine Learning
Chemical Physics
url https://arxiv.org/abs/2512.20924