A method for robust spin relaxometry in the presence of imperfect state preparation

Fuente: arXiv
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Bibliographic Details
Main Authors: Walsh, Ella P., Ahmadi, Sepehr, Healey, Alexander J., Simpson, David A., Hall, Liam T.
Format: Preprint
Published: 2025
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author Walsh, Ella P.
Ahmadi, Sepehr
Healey, Alexander J.
Simpson, David A.
Hall, Liam T.
author_facet Walsh, Ella P.
Ahmadi, Sepehr
Healey, Alexander J.
Simpson, David A.
Hall, Liam T.
contents Spin relaxometry based on quantum spin systems has developed as a valuable tool in medical and condensed matter systems, offering the advantage of operating without the need for external DC or RF fields. Spin relaxometry with nitrogen-vacancy (NV) centers has been applied to paramagnetic sensing using both single crystal diamond and nanodiamond materials. However, these methods often suffer from artifacts and systematic uncertainties, particularly due to imperfect spin state preparation, leading to artificially fast T$_1$ relaxation times. Current analysis techniques fail to adequately account for these issues, limiting the precision of parameter estimation. In this work, we introduce a minimal fitting procedure that enables more robust parameter estimation in the presence of imperfect spin polarization. Our model improves upon existing approaches by offering more accurate fits and provides a framework for efficiently parallelizing single-spin dynamics studies.
format Preprint
id arxiv_https___arxiv_org_abs_2512_22739
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle A method for robust spin relaxometry in the presence of imperfect state preparation
Walsh, Ella P.
Ahmadi, Sepehr
Healey, Alexander J.
Simpson, David A.
Hall, Liam T.
Quantum Physics
Spin relaxometry based on quantum spin systems has developed as a valuable tool in medical and condensed matter systems, offering the advantage of operating without the need for external DC or RF fields. Spin relaxometry with nitrogen-vacancy (NV) centers has been applied to paramagnetic sensing using both single crystal diamond and nanodiamond materials. However, these methods often suffer from artifacts and systematic uncertainties, particularly due to imperfect spin state preparation, leading to artificially fast T$_1$ relaxation times. Current analysis techniques fail to adequately account for these issues, limiting the precision of parameter estimation. In this work, we introduce a minimal fitting procedure that enables more robust parameter estimation in the presence of imperfect spin polarization. Our model improves upon existing approaches by offering more accurate fits and provides a framework for efficiently parallelizing single-spin dynamics studies.
title A method for robust spin relaxometry in the presence of imperfect state preparation
topic Quantum Physics
url https://arxiv.org/abs/2512.22739