Two-photon sweeping out of the K-shell of a heavy atomic ion

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Hauptverfasser: Hopersky, A. N., Nadolinsky, A. M., Novikov, S. A., Koneev, R. V.
Format: Preprint
Veröffentlicht: 2025
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author Hopersky, A. N.
Nadolinsky, A. M.
Novikov, S. A.
Koneev, R. V.
author_facet Hopersky, A. N.
Nadolinsky, A. M.
Novikov, S. A.
Koneev, R. V.
contents Within the framework of the second-order non-relativistic quantum perturbation theory, the methods of the theory of irreducible tensor operators, and nonorthogonal orbitals, the absolute values and shape of the generalized cross-sections of the two-photon double ionization (sweeping) of the K-shell of a heavy neon-like ion of an iron atom were predicted. The complete wave functions of the ground state of the ion and the states of its ionization are obtained in the single-configuration Hartree-Fock approximation. The effects of radial relaxation of ionization states in the field of one and two vacancies in the K-shell are taken into account. The matrix element of the operator of the radiation transition between continuum-spectrum states is taken into account by introducing a correlation function. It was established that the generalized cross-section of the two-photon sweeping of the K-shell at high (greater than or equal to 15.8 keV) energies of absorbed X-ray photons is several orders of magnitude greater than the generalized cross-section of the two-photon single ionization of the K-shell. This result qualitatively reproduces the work of Novikov S.A. and Hopersky A.N. (J. Phys. B 2002. V. 35. P. L339), stimulates future research, in particular, the effects of cascade "evaporation" of electron shells of an atom (atomic ion) when filling an empty K-shell and can be tested in X-ray free-electron laser experiments with high peak radiation brightness and ultrashort photon pulse duration. The scheme of the proposed experiment with two linearly polarized X-ray photons is presented.
format Preprint
id arxiv_https___arxiv_org_abs_2512_22896
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Two-photon sweeping out of the K-shell of a heavy atomic ion
Hopersky, A. N.
Nadolinsky, A. M.
Novikov, S. A.
Koneev, R. V.
Atomic Physics
00A81
Within the framework of the second-order non-relativistic quantum perturbation theory, the methods of the theory of irreducible tensor operators, and nonorthogonal orbitals, the absolute values and shape of the generalized cross-sections of the two-photon double ionization (sweeping) of the K-shell of a heavy neon-like ion of an iron atom were predicted. The complete wave functions of the ground state of the ion and the states of its ionization are obtained in the single-configuration Hartree-Fock approximation. The effects of radial relaxation of ionization states in the field of one and two vacancies in the K-shell are taken into account. The matrix element of the operator of the radiation transition between continuum-spectrum states is taken into account by introducing a correlation function. It was established that the generalized cross-section of the two-photon sweeping of the K-shell at high (greater than or equal to 15.8 keV) energies of absorbed X-ray photons is several orders of magnitude greater than the generalized cross-section of the two-photon single ionization of the K-shell. This result qualitatively reproduces the work of Novikov S.A. and Hopersky A.N. (J. Phys. B 2002. V. 35. P. L339), stimulates future research, in particular, the effects of cascade "evaporation" of electron shells of an atom (atomic ion) when filling an empty K-shell and can be tested in X-ray free-electron laser experiments with high peak radiation brightness and ultrashort photon pulse duration. The scheme of the proposed experiment with two linearly polarized X-ray photons is presented.
title Two-photon sweeping out of the K-shell of a heavy atomic ion
topic Atomic Physics
00A81
url https://arxiv.org/abs/2512.22896