A fluctuation-free pathway for a topological magnetic phase transition

Fuente: arXiv
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Main Authors: Battistelli, Riccardo, Körber, Lukas, Litzius, Kai, Grelier, Matthieu, Joy, Krishnanjana Puzhekadavil, Schneider, Michael, Wittrock, Steffen, Metternich, Daniel, Karaman, Tamer, Kern, Lisa-Marie, Klose, Christopher, Finizio, Simone, Fuchs, Josefin, Günther, Christian M., Butcher, Tim A., Prokeš, Karel, Boltje, Raluca, Patra, Manas, Wintz, Sebastian, Weigand, Markus, Petz, Sascha, Popescu, Horia, Raabe, Jörg, Jaouen, Nicolas, Eisebitt, Stefan, Cros, Vincent, Pfau, Bastian, Mentink, Johan H., Reyren, Nicolas, Büttner, Felix
Format: Preprint
Published: 2025
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author Battistelli, Riccardo
Körber, Lukas
Litzius, Kai
Grelier, Matthieu
Joy, Krishnanjana Puzhekadavil
Schneider, Michael
Wittrock, Steffen
Metternich, Daniel
Karaman, Tamer
Kern, Lisa-Marie
Klose, Christopher
Finizio, Simone
Fuchs, Josefin
Günther, Christian M.
Butcher, Tim A.
Prokeš, Karel
Boltje, Raluca
Patra, Manas
Wintz, Sebastian
Weigand, Markus
Petz, Sascha
Popescu, Horia
Raabe, Jörg
Jaouen, Nicolas
Eisebitt, Stefan
Cros, Vincent
Pfau, Bastian
Mentink, Johan H.
Reyren, Nicolas
Büttner, Felix
author_facet Battistelli, Riccardo
Körber, Lukas
Litzius, Kai
Grelier, Matthieu
Joy, Krishnanjana Puzhekadavil
Schneider, Michael
Wittrock, Steffen
Metternich, Daniel
Karaman, Tamer
Kern, Lisa-Marie
Klose, Christopher
Finizio, Simone
Fuchs, Josefin
Günther, Christian M.
Butcher, Tim A.
Prokeš, Karel
Boltje, Raluca
Patra, Manas
Wintz, Sebastian
Weigand, Markus
Petz, Sascha
Popescu, Horia
Raabe, Jörg
Jaouen, Nicolas
Eisebitt, Stefan
Cros, Vincent
Pfau, Bastian
Mentink, Johan H.
Reyren, Nicolas
Büttner, Felix
contents Topological magnetic textures are particle-like spin configurations stabilized by competing interactions. Their formation is commonly attributed to fluctuation-driven, first-order nucleation processes requiring activation over a topological energy barrier. Here, we demonstrate an alternative barrier- and fluctuation-free pathway for nucleating topological magnetic textures, triggered in our experiments by an excitation-induced spin reorientation transition. By combining x-ray imaging, scattering and micromagnetic simulations, we show that the system follows a deterministic cascade of symmetry-breaking phase transitions after excitation. First, the system undergoes a second-order phase transition from a homogeneous state to weak stripe domains, then a first-order transition to topologically trivial bubbles, and finally a topological switching event into skyrmionic textures. Through simulations, we generalize our findings and demonstrate that this pathway is active in a vast range of low-anisotropy materials. This previously unrecognized, spontaneous transition pathway suggests strategies for rapid, low-energy generation of topological spin textures and points to a general role of intrinsic modulational instabilities in phase transitions beyond magnetism.
format Preprint
id arxiv_https___arxiv_org_abs_2512_22947
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle A fluctuation-free pathway for a topological magnetic phase transition
Battistelli, Riccardo
Körber, Lukas
Litzius, Kai
Grelier, Matthieu
Joy, Krishnanjana Puzhekadavil
Schneider, Michael
Wittrock, Steffen
Metternich, Daniel
Karaman, Tamer
Kern, Lisa-Marie
Klose, Christopher
Finizio, Simone
Fuchs, Josefin
Günther, Christian M.
Butcher, Tim A.
Prokeš, Karel
Boltje, Raluca
Patra, Manas
Wintz, Sebastian
Weigand, Markus
Petz, Sascha
Popescu, Horia
Raabe, Jörg
Jaouen, Nicolas
Eisebitt, Stefan
Cros, Vincent
Pfau, Bastian
Mentink, Johan H.
Reyren, Nicolas
Büttner, Felix
Materials Science
Topological magnetic textures are particle-like spin configurations stabilized by competing interactions. Their formation is commonly attributed to fluctuation-driven, first-order nucleation processes requiring activation over a topological energy barrier. Here, we demonstrate an alternative barrier- and fluctuation-free pathway for nucleating topological magnetic textures, triggered in our experiments by an excitation-induced spin reorientation transition. By combining x-ray imaging, scattering and micromagnetic simulations, we show that the system follows a deterministic cascade of symmetry-breaking phase transitions after excitation. First, the system undergoes a second-order phase transition from a homogeneous state to weak stripe domains, then a first-order transition to topologically trivial bubbles, and finally a topological switching event into skyrmionic textures. Through simulations, we generalize our findings and demonstrate that this pathway is active in a vast range of low-anisotropy materials. This previously unrecognized, spontaneous transition pathway suggests strategies for rapid, low-energy generation of topological spin textures and points to a general role of intrinsic modulational instabilities in phase transitions beyond magnetism.
title A fluctuation-free pathway for a topological magnetic phase transition
topic Materials Science
url https://arxiv.org/abs/2512.22947