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Main Authors: Mottin, Stéphane, Świątkowska-Warkocka, Żaneta, Wolny-Marszałek, Marta, Itina, Tatiana E
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2512.23256
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author Mottin, Stéphane
Świątkowska-Warkocka, Żaneta
Wolny-Marszałek, Marta
Itina, Tatiana E
author_facet Mottin, Stéphane
Świątkowska-Warkocka, Żaneta
Wolny-Marszałek, Marta
Itina, Tatiana E
contents The interplay between laser parameters and liquid environments dictates the outcome of femtosecond laser-induced nanoparticle modification. We present a study of gold and iron oxide nanoparticles in water and a water-acetone mixture, irradiated with femtosecond lasers at 808 nm and 404 nm. While aggregation was observed in pure water at both wavelengths, the results revealed a strong stability and a rather unexpected wavelength-dependency in the acetone-water mixture. In this case, 808 nm irradiation produced some decrease in nanoparticle sizes, while 404 nm led to some nanoparticle growth. As a result, the acetone effect is found to be twofold: (i) on one hand, it helps to prevent aggregation; (ii) on the other hand, it acts as a reactive medium allowing to tune the nanoparticle size and composition simply by changing laser wavelength. So, this work emphasizes that solvent physical properties as well as laser-induced chemical processes in the solvent are not merely secondary effects but can dominate the final morphological outcome, providing a predictive framework for nanoparticle synthesis.
format Preprint
id arxiv_https___arxiv_org_abs_2512_23256
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Unveiling Solvent Effects on Femtosecond Laser-Irradiated Au/Fe3O4 Colloidal Nanoparticles: The Acetone Effect
Mottin, Stéphane
Świątkowska-Warkocka, Żaneta
Wolny-Marszałek, Marta
Itina, Tatiana E
Materials Science
The interplay between laser parameters and liquid environments dictates the outcome of femtosecond laser-induced nanoparticle modification. We present a study of gold and iron oxide nanoparticles in water and a water-acetone mixture, irradiated with femtosecond lasers at 808 nm and 404 nm. While aggregation was observed in pure water at both wavelengths, the results revealed a strong stability and a rather unexpected wavelength-dependency in the acetone-water mixture. In this case, 808 nm irradiation produced some decrease in nanoparticle sizes, while 404 nm led to some nanoparticle growth. As a result, the acetone effect is found to be twofold: (i) on one hand, it helps to prevent aggregation; (ii) on the other hand, it acts as a reactive medium allowing to tune the nanoparticle size and composition simply by changing laser wavelength. So, this work emphasizes that solvent physical properties as well as laser-induced chemical processes in the solvent are not merely secondary effects but can dominate the final morphological outcome, providing a predictive framework for nanoparticle synthesis.
title Unveiling Solvent Effects on Femtosecond Laser-Irradiated Au/Fe3O4 Colloidal Nanoparticles: The Acetone Effect
topic Materials Science
url https://arxiv.org/abs/2512.23256