Evidence for rare-region physics in the structural and electronic degrees of freedom of the nickelate La$_{2-x}$Sr$_x$NiO$_4$

Fuente: arXiv
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Main Authors: Spieker, R. J., Krohnke, B., Zhai, D., Benet, A. Lopez, Spaić, M., He, X., Tan, C. Y., Anderson, Z. W., Ye, F., Cao, H., Krogstad, M. J., Osborn, R., Pelc, D., Greven, M.
Format: Preprint
Published: 2025
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author Spieker, R. J.
Krohnke, B.
Zhai, D.
Benet, A. Lopez
Spaić, M.
He, X.
Tan, C. Y.
Anderson, Z. W.
Ye, F.
Cao, H.
Krogstad, M. J.
Osborn, R.
Pelc, D.
Greven, M.
author_facet Spieker, R. J.
Krohnke, B.
Zhai, D.
Benet, A. Lopez
Spaić, M.
He, X.
Tan, C. Y.
Anderson, Z. W.
Ye, F.
Cao, H.
Krogstad, M. J.
Osborn, R.
Pelc, D.
Greven, M.
contents We present a diffuse neutron and x-ray scattering study of structural, spin- and charge-density-wave fluctuations in the electrical insulator La$_{2-x}$Sr$_x$NiO$_4$. This lamellar nickelate is an isostructural analogue of the high-temperature cuprate superconductor La$_{2-x}$Sr$_x$CuO$_4$, for which recent experiments uncovered evidence for unusual structural and superconducting fluctuations indicative of rare-region physics due to inherent inhomogeneity unrelated to common point disorder effects. We find closely analogous nanoscale orthorhombic fluctuation behavior in La$_{2-x}$Sr$_x$NiO$_4$, including exponential scaling of the diffuse scattering intensity and power-law scaling of the characteristic length with relative temperature. Moreover, our neutron and x-ray scattering data reveal similar behavior for short-range magnetic and charge fluctuations above the respective ordering temperatures. These observations indicate that rare-region effects are a generic feature of perovskite-related structures and lead to universal fluctuations of both structural and electronic degrees of freedom over extended temperature ranges.
format Preprint
id arxiv_https___arxiv_org_abs_2512_23655
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Evidence for rare-region physics in the structural and electronic degrees of freedom of the nickelate La$_{2-x}$Sr$_x$NiO$_4$
Spieker, R. J.
Krohnke, B.
Zhai, D.
Benet, A. Lopez
Spaić, M.
He, X.
Tan, C. Y.
Anderson, Z. W.
Ye, F.
Cao, H.
Krogstad, M. J.
Osborn, R.
Pelc, D.
Greven, M.
Strongly Correlated Electrons
We present a diffuse neutron and x-ray scattering study of structural, spin- and charge-density-wave fluctuations in the electrical insulator La$_{2-x}$Sr$_x$NiO$_4$. This lamellar nickelate is an isostructural analogue of the high-temperature cuprate superconductor La$_{2-x}$Sr$_x$CuO$_4$, for which recent experiments uncovered evidence for unusual structural and superconducting fluctuations indicative of rare-region physics due to inherent inhomogeneity unrelated to common point disorder effects. We find closely analogous nanoscale orthorhombic fluctuation behavior in La$_{2-x}$Sr$_x$NiO$_4$, including exponential scaling of the diffuse scattering intensity and power-law scaling of the characteristic length with relative temperature. Moreover, our neutron and x-ray scattering data reveal similar behavior for short-range magnetic and charge fluctuations above the respective ordering temperatures. These observations indicate that rare-region effects are a generic feature of perovskite-related structures and lead to universal fluctuations of both structural and electronic degrees of freedom over extended temperature ranges.
title Evidence for rare-region physics in the structural and electronic degrees of freedom of the nickelate La$_{2-x}$Sr$_x$NiO$_4$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2512.23655