Pathway to Optical-Cycle Dynamic Photonics: Extreme Electron Temperatures in Transparent Conducting Oxides

Fuente: arXiv
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Main Authors: Choi, Jae Ik, Mkhitaryan, Vahagn, Fruhling, Colton, Khurgin, Jacob B., Kildishev, Alexander V., Shalaev, Vladimir M., Boltasseva, Alexandra
Format: Preprint
Published: 2025
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author Choi, Jae Ik
Mkhitaryan, Vahagn
Fruhling, Colton
Khurgin, Jacob B.
Kildishev, Alexander V.
Shalaev, Vladimir M.
Boltasseva, Alexandra
author_facet Choi, Jae Ik
Mkhitaryan, Vahagn
Fruhling, Colton
Khurgin, Jacob B.
Kildishev, Alexander V.
Shalaev, Vladimir M.
Boltasseva, Alexandra
contents We find that transparent conducting oxides (TCOs) exhibit oscillatory (sign-reversing) dynamics on a few optical cycle timescale under extreme electron temperatures. We demonstrate a mechanism for such transient dynamics and present an inverse-designed multilayer cavity incorporating an ultrathin TCO layer that supports the oscillatory behavior. This approach yields transmittance oscillations with a period of ~20 fs, which corresponds to three optical cycles of the probe beam. To achieve a similar oscillatory modulation in the refractive index, we incorporate a TCO electron-acceptor layer on top of the inverse-designed cavity, enabling thermionic carrier injection at the TCO heterojunction. The resulting acceptor layer achieves a striking Δn response time as short as 9 fs, approaching a single optical cycle, and is further tunable to sub-cycle timescales. The findings not only clarify the elusive transient physics in TCOs but also demonstrate, for the first time, the critical role of electron temperatures in driving oscillatory dynamic responses. More broadly, we establish TCO-based thermionic carrier injection as a practical route to novel time-varying photonic media operating on the timescale of an optical cycle, enabling time-reflection, time-refraction, and related dynamic phenomena from the visible to the infrared.
format Preprint
id arxiv_https___arxiv_org_abs_2512_24641
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Pathway to Optical-Cycle Dynamic Photonics: Extreme Electron Temperatures in Transparent Conducting Oxides
Choi, Jae Ik
Mkhitaryan, Vahagn
Fruhling, Colton
Khurgin, Jacob B.
Kildishev, Alexander V.
Shalaev, Vladimir M.
Boltasseva, Alexandra
Optics
We find that transparent conducting oxides (TCOs) exhibit oscillatory (sign-reversing) dynamics on a few optical cycle timescale under extreme electron temperatures. We demonstrate a mechanism for such transient dynamics and present an inverse-designed multilayer cavity incorporating an ultrathin TCO layer that supports the oscillatory behavior. This approach yields transmittance oscillations with a period of ~20 fs, which corresponds to three optical cycles of the probe beam. To achieve a similar oscillatory modulation in the refractive index, we incorporate a TCO electron-acceptor layer on top of the inverse-designed cavity, enabling thermionic carrier injection at the TCO heterojunction. The resulting acceptor layer achieves a striking Δn response time as short as 9 fs, approaching a single optical cycle, and is further tunable to sub-cycle timescales. The findings not only clarify the elusive transient physics in TCOs but also demonstrate, for the first time, the critical role of electron temperatures in driving oscillatory dynamic responses. More broadly, we establish TCO-based thermionic carrier injection as a practical route to novel time-varying photonic media operating on the timescale of an optical cycle, enabling time-reflection, time-refraction, and related dynamic phenomena from the visible to the infrared.
title Pathway to Optical-Cycle Dynamic Photonics: Extreme Electron Temperatures in Transparent Conducting Oxides
topic Optics
url https://arxiv.org/abs/2512.24641