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Bibliographische Detailangaben
Hauptverfasser: Fukami, Kai, Shoji, Eita
Format: Preprint
Veröffentlicht: 2026
Schlagworte:
Online-Zugang:https://arxiv.org/abs/2601.01776
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Inhaltsangabe:
  • Superspreading wetting is traditionally attributed to surfactant-driven mechanisms. However, recent observations of superspreading in surfactant-free nanofluids defy standard theoretical explanations. This study considers a data-driven approach to model droplet dynamics with the thickness of liquid films on the nanometer-micrometer scale in a compact form of a partial differential equation. We examine spatiotemporal film-thickness profiles resolved at the nanometer scale via phase-shifting imaging ellipsometry. For a pure solvent, the present governing equation recovers the classical lubrication physics driven by disjoining pressure and evaporation. In contrast, the nanofluid dynamics necessitates a unique transport term scaling with the gradient of the inverse film thickness. Theoretical analysis suggests this term represents a nanoparticle-induced bias flux, consistent with a hypothesized capillary wicking mechanism within the precursor film. The identification of the current nanofluid-specific term underscores the efficacy of integrating high-precision experimental measurements with data-driven modeling to unravel complex wetting dynamics.