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Detalles Bibliográficos
Autores principales: Huet, X., Aerts, A., Vaeck, N., Génévriez, M., Urbain, X.
Formato: Preprint
Publicado: 2026
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Acceso en línea:https://arxiv.org/abs/2601.01933
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  • We report rovibronic spectra of the A $^3Σ^+$($v'=0-2$) - X $^3Π_Ω(v=0)$ rovibronic transitions ($|Ω|=0, 1$ and 2) of the CO$^{2+}$ doubly-charged molecular ion. Spectra were recorded at high resolution ($\sim 5$~cm$^{-1}$) in a fast beam of CO$^{2+}$ molecules by detecting the Coulomb explosion of the molecules upon excitation to the A state. Measurements were guided by \textit{ab initio} calculations which then assisted the assignment of the observed spectral features. Our results resolve the spin-orbit splittings of the ground vibronic state X $^3Π_Ω(v=0)$, but not the rotational structure of the bands due to spectral congestion, and provide spectroscopic information on CO$^{2+}$ with unprecedented resolution. In doing so they expand our knowledge of this benchmark doubly charged molecular ion and expand the short list of doubly charged molecules studied at high resolution.