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Bibliographic Details
Main Authors: Pierron, Thomas, Castro, José de Jesùs Villalobos, Barre, Etienne, Wang, Dan, Pons, Stephane, Roditchev, Dimitri, Bendounan, Azzedine, Guisset, Valerie, David, Philippe, Coraux, Johann, Sponza, Lorenzo, Vlaic, Sergio
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2601.02922
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Table of Contents:
  • The electronic properties of the two-dimensional (2D) $α$ phase of antimonene are unique, featuring unpinned Dirac cones that can be moved with strain. Here we investigate the structural and electronic properties of an epitaxial 2D $α$-antimonene, grown on Au(111). Using angle-resolved photoemission spectroscopy and density-functional theory, we reveal a strong hybridization at the Sb/Au interface, which imprints a rectangular reconstruction in the Au states, producing a band folding and hybrid bands exhibiting trigonal pockets. Additionally, hybridization displaces part of the Au wavefunction in regions of large electrostatic potential gradient, thereby enhancing spin-orbit splitting. Our work underscores that the pristine electronic properties of $α$-antimonene may be deeply modified by its substrate, and even overwhelmed by the bands of the latter, and also shows that spin-orbit interaction in a heavy metal (Au) can be substantially enhanced by a lighter element (Sb).