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Main Authors: Wu, Jianyu, Niedermayr, Arthur, Cao, Gaolong, Grånäs, Oscar, Weissenrieder, Jonas
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2601.03881
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author Wu, Jianyu
Niedermayr, Arthur
Cao, Gaolong
Grånäs, Oscar
Weissenrieder, Jonas
author_facet Wu, Jianyu
Niedermayr, Arthur
Cao, Gaolong
Grånäs, Oscar
Weissenrieder, Jonas
contents Microscopic and dynamic control over quantum states is essential for bridging fundamental studies of material properties to device function. Realizing such control at combined high spatial resolution and ultrafast temporal precision remains a major challenge. Here, we demonstrate femtosecond laser-driven patterning of topological quantum states in the Weyl semimetal WTe2. By engineering the excitation field into a transient optical grating, we spatially selectively and reversibly drive phase transitions between the topological Td and topologically trivial 1T* phases. Using ultrafast transmission electron microscopy, we directly visualize the formation of a periodic Td/1T* heterostructure, observe the propagation of a phase front, and analyze nanoscale confinement of coherently excited optical phonon modes. Our findings establish a platform for all-optical, spatially programmable, and reconfigurable control of quantum states, paving the way for optically addressable topological devices.
format Preprint
id arxiv_https___arxiv_org_abs_2601_03881
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Ultrafast laser-driven topological phase patterning
Wu, Jianyu
Niedermayr, Arthur
Cao, Gaolong
Grånäs, Oscar
Weissenrieder, Jonas
Materials Science
Microscopic and dynamic control over quantum states is essential for bridging fundamental studies of material properties to device function. Realizing such control at combined high spatial resolution and ultrafast temporal precision remains a major challenge. Here, we demonstrate femtosecond laser-driven patterning of topological quantum states in the Weyl semimetal WTe2. By engineering the excitation field into a transient optical grating, we spatially selectively and reversibly drive phase transitions between the topological Td and topologically trivial 1T* phases. Using ultrafast transmission electron microscopy, we directly visualize the formation of a periodic Td/1T* heterostructure, observe the propagation of a phase front, and analyze nanoscale confinement of coherently excited optical phonon modes. Our findings establish a platform for all-optical, spatially programmable, and reconfigurable control of quantum states, paving the way for optically addressable topological devices.
title Ultrafast laser-driven topological phase patterning
topic Materials Science
url https://arxiv.org/abs/2601.03881