Coexistence of long-range magnetic order and dynamical magnetism in the V-based Kagome metals: A combined thermodynamic and $μ$SR study

Fuente: arXiv
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Autori principali: Devi, Sheetal, Zhou, Yishui, Hicken, Thomas J., Guguchia, Zurab, Luetkens, Hubertus, Lee, Min-Kai, Chang, Lieh-Jeng, Su, Yixi
Natura: Preprint
Pubblicazione: 2026
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author Devi, Sheetal
Zhou, Yishui
Hicken, Thomas J.
Guguchia, Zurab
Luetkens, Hubertus
Lee, Min-Kai
Chang, Lieh-Jeng
Su, Yixi
author_facet Devi, Sheetal
Zhou, Yishui
Hicken, Thomas J.
Guguchia, Zurab
Luetkens, Hubertus
Lee, Min-Kai
Chang, Lieh-Jeng
Su, Yixi
contents V-based Kagome metals exhibit a unique lattice geometry that can give rise to exotic electronic and magnetic phenomena, making them an ideal platform to study the interplay of topology and magnetism. We present a combined thermodynamic and muon spin relaxation ($μ$SR) investigation of single-crystal RV$_{6}$Sn$_{6}$ (R = Tb, Dy, Ho, Er) compounds, focusing on their low-temperature magnetic behavior. Heat capacity and $μ$SR measurements reveal distinct magnetic phase transitions below 4 K, confirming the emergence of long-range magnetic order in all compounds studied. The $μ$SR results further indicate persistent spin fluctuations within the magnetically ordered state down to 50 mK, reflected in reduced ordered moments obtained from hyperfine analysis of the heat capacity measurements. These findings uncover the coexistence of static and dynamic magnetism in V-based Kagome metals and emphasizing the key role of 4$f$-electron anisotropy in shaping their magnetic ground states. Compared with the Mn-based RMn$_{6}$Sn$_{6}$ analogs, our results highlight the unique magnetism arising from the decoupled rare-earth sublattice and its interplay with the nonmagnetic V Kagome network.
format Preprint
id arxiv_https___arxiv_org_abs_2601_09046
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Coexistence of long-range magnetic order and dynamical magnetism in the V-based Kagome metals: A combined thermodynamic and $μ$SR study
Devi, Sheetal
Zhou, Yishui
Hicken, Thomas J.
Guguchia, Zurab
Luetkens, Hubertus
Lee, Min-Kai
Chang, Lieh-Jeng
Su, Yixi
Strongly Correlated Electrons
V-based Kagome metals exhibit a unique lattice geometry that can give rise to exotic electronic and magnetic phenomena, making them an ideal platform to study the interplay of topology and magnetism. We present a combined thermodynamic and muon spin relaxation ($μ$SR) investigation of single-crystal RV$_{6}$Sn$_{6}$ (R = Tb, Dy, Ho, Er) compounds, focusing on their low-temperature magnetic behavior. Heat capacity and $μ$SR measurements reveal distinct magnetic phase transitions below 4 K, confirming the emergence of long-range magnetic order in all compounds studied. The $μ$SR results further indicate persistent spin fluctuations within the magnetically ordered state down to 50 mK, reflected in reduced ordered moments obtained from hyperfine analysis of the heat capacity measurements. These findings uncover the coexistence of static and dynamic magnetism in V-based Kagome metals and emphasizing the key role of 4$f$-electron anisotropy in shaping their magnetic ground states. Compared with the Mn-based RMn$_{6}$Sn$_{6}$ analogs, our results highlight the unique magnetism arising from the decoupled rare-earth sublattice and its interplay with the nonmagnetic V Kagome network.
title Coexistence of long-range magnetic order and dynamical magnetism in the V-based Kagome metals: A combined thermodynamic and $μ$SR study
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2601.09046