Unexpected type-II multiferroic phase in GdMnO3 under high magnetic fields

Fuente: arXiv
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Hauptverfasser: Yang, Ming, Chen, Jun, Wang, Junfeng, Dong, Chao, Lu, Chengliang, Xu, Gang, Cheng, Jinguang, Zhou, Jianshi, Dong, Shuai
Format: Preprint
Veröffentlicht: 2026
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author Yang, Ming
Chen, Jun
Wang, Junfeng
Dong, Chao
Lu, Chengliang
Xu, Gang
Cheng, Jinguang
Zhou, Jianshi
Dong, Shuai
author_facet Yang, Ming
Chen, Jun
Wang, Junfeng
Dong, Chao
Lu, Chengliang
Xu, Gang
Cheng, Jinguang
Zhou, Jianshi
Dong, Shuai
contents Perovskite manganites with small A-site ions, as the first and canonical branch of type-II multiferroics, are ideal systems to exhibit magnetism-induced ferroelectricity. Despite their established magnetoelectric phase diagrams under low magnetic fields, here an unidentified phase with a large magnetism-induced polarization (up to 1500 μC/m2) is revealed in GdMnO3 under high magnetic fields up to 60 T. Based on multiprobe experiments, a complete phase diagram is constructed with successive polar-nonpolar-polar-nonpolar transitions. Such a nonmonotonic evolution is well mimicked by model simulation, while the spin-lattice coupling is the key ingredient for the reentrant ferroelectric phase.
format Preprint
id arxiv_https___arxiv_org_abs_2601_09092
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Unexpected type-II multiferroic phase in GdMnO3 under high magnetic fields
Yang, Ming
Chen, Jun
Wang, Junfeng
Dong, Chao
Lu, Chengliang
Xu, Gang
Cheng, Jinguang
Zhou, Jianshi
Dong, Shuai
Materials Science
Perovskite manganites with small A-site ions, as the first and canonical branch of type-II multiferroics, are ideal systems to exhibit magnetism-induced ferroelectricity. Despite their established magnetoelectric phase diagrams under low magnetic fields, here an unidentified phase with a large magnetism-induced polarization (up to 1500 μC/m2) is revealed in GdMnO3 under high magnetic fields up to 60 T. Based on multiprobe experiments, a complete phase diagram is constructed with successive polar-nonpolar-polar-nonpolar transitions. Such a nonmonotonic evolution is well mimicked by model simulation, while the spin-lattice coupling is the key ingredient for the reentrant ferroelectric phase.
title Unexpected type-II multiferroic phase in GdMnO3 under high magnetic fields
topic Materials Science
url https://arxiv.org/abs/2601.09092