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Main Authors: Gu, Yaohui, Li, Binbo, Jiang, Lingyang, Hu, Yuhui, Liu, Wenqiang, Xu, Lijun, Zhai, Pengfei, Liu, Jie, Duan, Jinglai
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2601.10174
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author Gu, Yaohui
Li, Binbo
Jiang, Lingyang
Hu, Yuhui
Liu, Wenqiang
Xu, Lijun
Zhai, Pengfei
Liu, Jie
Duan, Jinglai
author_facet Gu, Yaohui
Li, Binbo
Jiang, Lingyang
Hu, Yuhui
Liu, Wenqiang
Xu, Lijun
Zhai, Pengfei
Liu, Jie
Duan, Jinglai
contents Gallium oxide (Ga2O3) is a wide-bandgap semiconductor with promising applications in high-power and high-frequency electronics. However, its complex polymorphic nature poses substantial challenges for fundamental studies, particularly in understanding phase-transformation behaviors under nonequilibrium conditions. Here, we develop a robust, accurate, and computationally efficient machine-learning interatomic potential (MLIP) for Ga2O3 based on the neuroevolution potential (NEP) framework combined with an energy-dependent weighting strategy. The resulting NEP potential demonstrates clear advantages over the state-of-the-art tabGAP potential with respect to both accuracy and computational efficiency. Furthermore, we introduce a physically process-oriented sampling strategy to systematically augment the training dataset, thereby enhancing the MLIP performance for targeted physical phenomena. As a representative application, a dedicated NEP potential is constructed for swift heavy-ion (SHI) irradiation simulations of \b{eta}-Ga2O3. The simulated results are in quantitative agreement with experimental observations and provide a consistent physical explanation for the reported experimental discrepancies regarding phase transformations in the ion track of \b{eta}-Ga2O3.
format Preprint
id arxiv_https___arxiv_org_abs_2601_10174
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle A Neuroevolution Potential for Gallium Oxide: Accurate and Efficient Modeling of Polymorphism and Swift Heavy-Ion Irradiation
Gu, Yaohui
Li, Binbo
Jiang, Lingyang
Hu, Yuhui
Liu, Wenqiang
Xu, Lijun
Zhai, Pengfei
Liu, Jie
Duan, Jinglai
Materials Science
Gallium oxide (Ga2O3) is a wide-bandgap semiconductor with promising applications in high-power and high-frequency electronics. However, its complex polymorphic nature poses substantial challenges for fundamental studies, particularly in understanding phase-transformation behaviors under nonequilibrium conditions. Here, we develop a robust, accurate, and computationally efficient machine-learning interatomic potential (MLIP) for Ga2O3 based on the neuroevolution potential (NEP) framework combined with an energy-dependent weighting strategy. The resulting NEP potential demonstrates clear advantages over the state-of-the-art tabGAP potential with respect to both accuracy and computational efficiency. Furthermore, we introduce a physically process-oriented sampling strategy to systematically augment the training dataset, thereby enhancing the MLIP performance for targeted physical phenomena. As a representative application, a dedicated NEP potential is constructed for swift heavy-ion (SHI) irradiation simulations of \b{eta}-Ga2O3. The simulated results are in quantitative agreement with experimental observations and provide a consistent physical explanation for the reported experimental discrepancies regarding phase transformations in the ion track of \b{eta}-Ga2O3.
title A Neuroevolution Potential for Gallium Oxide: Accurate and Efficient Modeling of Polymorphism and Swift Heavy-Ion Irradiation
topic Materials Science
url https://arxiv.org/abs/2601.10174