Revealing mesoscale bubble and particle dynamics in ultrasound-driven multiphase fluids by ultrafast synchrotron X-ray radiography and hybrid modelling

Fuente: arXiv
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Main Authors: Qin, Ling, Xiang, Kang, Tzanakis, Iakovos, Eskin, Dmitry, Clark, Samuel, Fezzaa, Kamel, Mi, Jiawei
Format: Preprint
Published: 2026
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author Qin, Ling
Xiang, Kang
Tzanakis, Iakovos
Eskin, Dmitry
Clark, Samuel
Fezzaa, Kamel
Mi, Jiawei
author_facet Qin, Ling
Xiang, Kang
Tzanakis, Iakovos
Eskin, Dmitry
Clark, Samuel
Fezzaa, Kamel
Mi, Jiawei
contents Multiphase fluid flows comprising of mesoscale solid particles, liquid droplets, or gas bubbles are common in both natural and man-made systems, but quantifying the energy transfer is challenging due to complex bubble-particle interactions. In this study, we used ultrafast synchrotron X-ray imaging to study the mesoscale dynamic interactions among ultrasonic cavitation bubbles and hydrophobic particles or clusters. Critical dynamic information and data were extracted from the vast amount of X-ray images and then fed into the hybrid analytical-numerical model for calculating the energy transfer from the oscillating bubble and the imploding bubble to the nearby hydrophobic particles. Using the Ni spherical microparticles as an example, at bubble oscillation approximately 16% (80-320 nJ) of the local energy was transferred to the particle. At bubble implosion, the transferred energy increased approximately 26% (0.135-1.09 uJ). Local energy transfer occurred on timescales of 1 us to 1 ms and length scales of 1 um to 1 mm. Within each ultrasound cycle, kinetic and potential energy underwent complex exchanges, with local energy exhibiting a stepwise decay at the end of each cycle. The transferred energy was mainly consumed for enabling highly efficient particle dispersion. This research provides quantitative insights into optimizing hydrophobic nanomaterial dispersion and has broader implications for interfacial energy transfer processes such as making suspensions, composite materials and exfoliated 2D materials.
format Preprint
id arxiv_https___arxiv_org_abs_2601_13582
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Revealing mesoscale bubble and particle dynamics in ultrasound-driven multiphase fluids by ultrafast synchrotron X-ray radiography and hybrid modelling
Qin, Ling
Xiang, Kang
Tzanakis, Iakovos
Eskin, Dmitry
Clark, Samuel
Fezzaa, Kamel
Mi, Jiawei
Fluid Dynamics
Mesoscale and Nanoscale Physics
Multiphase fluid flows comprising of mesoscale solid particles, liquid droplets, or gas bubbles are common in both natural and man-made systems, but quantifying the energy transfer is challenging due to complex bubble-particle interactions. In this study, we used ultrafast synchrotron X-ray imaging to study the mesoscale dynamic interactions among ultrasonic cavitation bubbles and hydrophobic particles or clusters. Critical dynamic information and data were extracted from the vast amount of X-ray images and then fed into the hybrid analytical-numerical model for calculating the energy transfer from the oscillating bubble and the imploding bubble to the nearby hydrophobic particles. Using the Ni spherical microparticles as an example, at bubble oscillation approximately 16% (80-320 nJ) of the local energy was transferred to the particle. At bubble implosion, the transferred energy increased approximately 26% (0.135-1.09 uJ). Local energy transfer occurred on timescales of 1 us to 1 ms and length scales of 1 um to 1 mm. Within each ultrasound cycle, kinetic and potential energy underwent complex exchanges, with local energy exhibiting a stepwise decay at the end of each cycle. The transferred energy was mainly consumed for enabling highly efficient particle dispersion. This research provides quantitative insights into optimizing hydrophobic nanomaterial dispersion and has broader implications for interfacial energy transfer processes such as making suspensions, composite materials and exfoliated 2D materials.
title Revealing mesoscale bubble and particle dynamics in ultrasound-driven multiphase fluids by ultrafast synchrotron X-ray radiography and hybrid modelling
topic Fluid Dynamics
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2601.13582