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Main Authors: Fujimaru, Tomoyasu, Hirai, Kanta, Inamata, Masato, Tanaka, Hiromu, Ikeuchi, Midori, Yamashita, Hidehiro, Haruta, Mitsutaka, Tamaoka, Takehiko, Kawasaki, Naohiko, Saito, Hikaru
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2601.14898
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author Fujimaru, Tomoyasu
Hirai, Kanta
Inamata, Masato
Tanaka, Hiromu
Ikeuchi, Midori
Yamashita, Hidehiro
Haruta, Mitsutaka
Tamaoka, Takehiko
Kawasaki, Naohiko
Saito, Hikaru
author_facet Fujimaru, Tomoyasu
Hirai, Kanta
Inamata, Masato
Tanaka, Hiromu
Ikeuchi, Midori
Yamashita, Hidehiro
Haruta, Mitsutaka
Tamaoka, Takehiko
Kawasaki, Naohiko
Saito, Hikaru
contents Integration of high-quality photon emitters at specific locations within nanophotonic structures or optoelectronic devices is a key to innovating on-chip optical control and quantum technologies. Halide perovskite nanoparticles have great potential as single photon emitters with high quantum efficiency. To achieve their full potential, they must be embedded in a host material that ensures chemical stability and passivates surface defects. A previous experiment on a CsPbBr3-Cs4PbBr6 nanocomposite film suggested possibility that electron beam irradiation can be used to control positions of CsPbBr3 nano-light sources in the Cs4PbBr6 host although the effects of electron beam irradiation are not fully understood. Here, we fabricate a Cs4PbBr6-CsBr film, not containing the CsPbBr3 phase, and provide direct evidence that CsPbBr3 nanoparticles can be locally generated in the Cs4PbBr6 host by irradiation with a focused electron beam. We further demonstrate perovskite nano-light source arrays with submicron spacing using this method.
format Preprint
id arxiv_https___arxiv_org_abs_2601_14898
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Precisely positioned generation of CsPbBr3 nano-light sources in a Cs4PbBr6 film by electron beam irradiation
Fujimaru, Tomoyasu
Hirai, Kanta
Inamata, Masato
Tanaka, Hiromu
Ikeuchi, Midori
Yamashita, Hidehiro
Haruta, Mitsutaka
Tamaoka, Takehiko
Kawasaki, Naohiko
Saito, Hikaru
Mesoscale and Nanoscale Physics
Integration of high-quality photon emitters at specific locations within nanophotonic structures or optoelectronic devices is a key to innovating on-chip optical control and quantum technologies. Halide perovskite nanoparticles have great potential as single photon emitters with high quantum efficiency. To achieve their full potential, they must be embedded in a host material that ensures chemical stability and passivates surface defects. A previous experiment on a CsPbBr3-Cs4PbBr6 nanocomposite film suggested possibility that electron beam irradiation can be used to control positions of CsPbBr3 nano-light sources in the Cs4PbBr6 host although the effects of electron beam irradiation are not fully understood. Here, we fabricate a Cs4PbBr6-CsBr film, not containing the CsPbBr3 phase, and provide direct evidence that CsPbBr3 nanoparticles can be locally generated in the Cs4PbBr6 host by irradiation with a focused electron beam. We further demonstrate perovskite nano-light source arrays with submicron spacing using this method.
title Precisely positioned generation of CsPbBr3 nano-light sources in a Cs4PbBr6 film by electron beam irradiation
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2601.14898