Mid-infrared high-sensitive cavity-free in-situ CO gas sensing based on up-conversion detection

Fuente: arXiv
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Auteurs principaux: Han, Zhao-Qi-Zhi, Zhang, He, Yang, Fan, Wang, Xiao-Hua, Liu, Bo-Wen, Li, Jin-Peng, Zhou, Zheng-He, Li, Yin-Hai, Li, Yan, Zhou, Zhi-Yuan, Shi, Bao-Sen
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Publié: 2026
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author Han, Zhao-Qi-Zhi
Zhang, He
Yang, Fan
Wang, Xiao-Hua
Liu, Bo-Wen
Li, Jin-Peng
Zhou, Zheng-He
Li, Yin-Hai
Li, Yan
Zhou, Zhi-Yuan
Shi, Bao-Sen
author_facet Han, Zhao-Qi-Zhi
Zhang, He
Yang, Fan
Wang, Xiao-Hua
Liu, Bo-Wen
Li, Jin-Peng
Zhou, Zheng-He
Li, Yin-Hai
Li, Yan
Zhou, Zhi-Yuan
Shi, Bao-Sen
contents Carbon monoxide (CO) is a significant indicator gas with considerable application value in atmospheric monitoring, industrial production and medical diagnosis. Its fundamental vibrational band locates around 4.6 $\upmu$m and has larger absorption line strength than that of overtone band, which is more suitable for the precise identification and concentration detection of CO. In this paper, the up-conversion detection is employed to convert the mid-infrared absorption signal obtained by TDLAS to the visible light band, then a silicon-based detector is utilized for detection. By which, we can achieve the highest sensitivity of 79.6 ppb under the condition of cavity-free in-situ with an absorption range length of only 0.14 m. Furthermore, the single-photon level real-time detection of CO concentration after the diffuse reflection is realized by using SPAD. This work demonstrates the merits of the up-conversion detection in terms of its functionality at room temperature and capacity for sensitivity detection. Furthermore, it presents a design and optimization methodology that has the potential to underpin the advancement of the method towards more practical applications, like industrial process monitoring, medical diagnosis and so on.
format Preprint
id arxiv_https___arxiv_org_abs_2601_15981
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Mid-infrared high-sensitive cavity-free in-situ CO gas sensing based on up-conversion detection
Han, Zhao-Qi-Zhi
Zhang, He
Yang, Fan
Wang, Xiao-Hua
Liu, Bo-Wen
Li, Jin-Peng
Zhou, Zheng-He
Li, Yin-Hai
Li, Yan
Zhou, Zhi-Yuan
Shi, Bao-Sen
Optics
Instrumentation and Detectors
Carbon monoxide (CO) is a significant indicator gas with considerable application value in atmospheric monitoring, industrial production and medical diagnosis. Its fundamental vibrational band locates around 4.6 $\upmu$m and has larger absorption line strength than that of overtone band, which is more suitable for the precise identification and concentration detection of CO. In this paper, the up-conversion detection is employed to convert the mid-infrared absorption signal obtained by TDLAS to the visible light band, then a silicon-based detector is utilized for detection. By which, we can achieve the highest sensitivity of 79.6 ppb under the condition of cavity-free in-situ with an absorption range length of only 0.14 m. Furthermore, the single-photon level real-time detection of CO concentration after the diffuse reflection is realized by using SPAD. This work demonstrates the merits of the up-conversion detection in terms of its functionality at room temperature and capacity for sensitivity detection. Furthermore, it presents a design and optimization methodology that has the potential to underpin the advancement of the method towards more practical applications, like industrial process monitoring, medical diagnosis and so on.
title Mid-infrared high-sensitive cavity-free in-situ CO gas sensing based on up-conversion detection
topic Optics
Instrumentation and Detectors
url https://arxiv.org/abs/2601.15981