Reducing TLS loss in tantalum CPW resonators using titanium sacrificial layers

Fuente: arXiv
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Hauptverfasser: Degnan, Zachary, Chiu, Chun-Ching, Chen, Yi-Hsun, Sommers, David, Abdurakhimov, Leonid, Zhu, Lihuang, Fedorov, Arkady, Jacobson, Peter
Format: Preprint
Veröffentlicht: 2026
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author Degnan, Zachary
Chiu, Chun-Ching
Chen, Yi-Hsun
Sommers, David
Abdurakhimov, Leonid
Zhu, Lihuang
Fedorov, Arkady
Jacobson, Peter
author_facet Degnan, Zachary
Chiu, Chun-Ching
Chen, Yi-Hsun
Sommers, David
Abdurakhimov, Leonid
Zhu, Lihuang
Fedorov, Arkady
Jacobson, Peter
contents We demonstrate a substantial reduction in two-level system loss in tantalum coplanar waveguide resonators fabricated on high-resistivity silicon substrates through the use of an ultrathin titanium sacrificial layer. A 0.2nm titanium film, deposited atop pre-sputtered α-tantalum, acts as a solid-state oxygen getter that chemically modifies the native Ta oxide at the metal-air interface. After device fabrication, the titanium layer is removed using buffered oxide etchant, leaving behind a chemically reduced Ta oxide surface. Subsequent high-vacuum annealing further suppresses two-level system loss. Resonators treated with this process exhibit internal quality factors Qi exceeding an average of 1.5 million in the single-photon regime across ten devices, over three times higher than otherwise identical devices lacking the titanium layer. These results highlight the critical role of interfacial oxide chemistry in superconducting loss and reinforce atomic-scale surface engineering as an effective approach to improving coherence in tantalum-based quantum circuits. The method is compatible with existing fabrication workflows applicable to tantalum films, offering a practical route to further extending T1 lifetimes in superconducting qubits.
format Preprint
id arxiv_https___arxiv_org_abs_2601_16369
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Reducing TLS loss in tantalum CPW resonators using titanium sacrificial layers
Degnan, Zachary
Chiu, Chun-Ching
Chen, Yi-Hsun
Sommers, David
Abdurakhimov, Leonid
Zhu, Lihuang
Fedorov, Arkady
Jacobson, Peter
Quantum Physics
Materials Science
Superconductivity
We demonstrate a substantial reduction in two-level system loss in tantalum coplanar waveguide resonators fabricated on high-resistivity silicon substrates through the use of an ultrathin titanium sacrificial layer. A 0.2nm titanium film, deposited atop pre-sputtered α-tantalum, acts as a solid-state oxygen getter that chemically modifies the native Ta oxide at the metal-air interface. After device fabrication, the titanium layer is removed using buffered oxide etchant, leaving behind a chemically reduced Ta oxide surface. Subsequent high-vacuum annealing further suppresses two-level system loss. Resonators treated with this process exhibit internal quality factors Qi exceeding an average of 1.5 million in the single-photon regime across ten devices, over three times higher than otherwise identical devices lacking the titanium layer. These results highlight the critical role of interfacial oxide chemistry in superconducting loss and reinforce atomic-scale surface engineering as an effective approach to improving coherence in tantalum-based quantum circuits. The method is compatible with existing fabrication workflows applicable to tantalum films, offering a practical route to further extending T1 lifetimes in superconducting qubits.
title Reducing TLS loss in tantalum CPW resonators using titanium sacrificial layers
topic Quantum Physics
Materials Science
Superconductivity
url https://arxiv.org/abs/2601.16369